The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
CO2/N2 separations with mixed-matrix membranes containing Mg2(dobdc) nanocrystals
Abstract
Nanocrystals of M2(dobdc) (M = Mg, Ni, Zn; dobdc4− = 1,4-dioxido-2,5-benzenedicarboxylate), also known as M-MOF-74 or CPO-27-M, with diameters of ∼100 nm or less were synthesized using a room-temperature reaction of 2 h duration. Adsorption data collected for CO2 and N2 show slightly lower surface areas but similar adsorption selectivites relative to the bulk materials. High-quality mixed-matrix membranes containing Mg2(dobdc) nanocrystals were fabricated using three different polymers for testing under conditions relevant to the removal of CO2 from flue gas. Significant enhancements in CO2 permeability and CO2/N2 selectivity over a pure polymer membrane were observed when a glassy polyimide was employed as the matrix, while membranes made with rubbery polymers showed decreased permeabilities, presumably due to the plugging of Mg2(dobdc) pores by polymer chains having a high mobility at room temperature.
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Cites
Metal-organic framework materials as catalysts
Lee, J., Farha, O. K., Roberts, J., Scheidt, K. A., Nguyen, S. T., & Hupp, J. T. (2009) · Chemical Society Reviews · doi:10.1039/b807080f · Cited by 7,969
Cited by
Metal‐Organic Framework‐Based Nanomaterials for Electrocatalysis
Mahmood, A., Guo, W., Tabassum, H., & Zou, R. (2016) · Advanced Energy Materials · doi:10.1002/aenm.201600423 · Cited by 632
Advanced Porous Materials in Mixed Matrix Membranes
Cheng, Y., Ying, Y., Japip, S., Jiang, S., Chung, T., Zhang, S., & Zhao, D. (2018) · Advanced Materials · doi:10.1002/adma.201802401 · Cited by 448
Carbon Capture From Flue Gas and the Atmosphere: A Perspective
Wang, X., & Song, C. (2020) · Frontiers in Energy Research · doi:10.3389/fenrg.2020.560849 · Cited by 428
Advances in metal–organic framework-based membranes
Cheng, Y., Datta, S. J., Zhou, S., Jia, J., Shekhah, O., & Eddaoudi, M. (2022) · Chemical Society Reviews · doi:10.1039/d2cs00031h · Cited by 423
Zhang, R., Ji, S., Wang, N., Wang, L., Zhang, G., & Li, J. (2014) · Angewandte Chemie International Edition · doi:10.1002/anie.201403978 · Cited by 406
Metadata
- Authors
- Bae, T.-H., & Long, J. R.
- Venue
- Energy & Environmental Science
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2013
- Volume
- 6
- Issue
- 12
- Pages
- 3565
- ISSN
- 1754-5692 (ISSN-L)
- 1754-5706
- OpenAlex
- W2114889971
- Cited by
- 226
- References
- 1
- FWCI
- 22.58
- Type
- journal article
- Language
- en
- Open access
- closed
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- Bae, T.-H., & Long, J. R. (2013). CO2/N2 separations with mixed-matrix membranes containing Mg2(dobdc) nanocrystals. Energy & Environmental Science. https://doi.org/10.1039/c3ee42394h
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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