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Heterostructured Ag3PO4/AgBr/Ag plasmonic photocatalyst with enhanced photocatalytic activity and stability under visible light
Abstract
A heterostructured Ag3PO4/AgBr/Ag plasmonic photocatalyst was prepared by a rational in situ ion exchange reaction between Ag3PO4 micro-cubes and Br(-) in aqueous solution followed by photoreduction. The photocatalytic activities of obtained photocatalysts were measured by the degradation of methyl orange (MO) and methylene blue (MB) under visible light irradiation (λ≥ 400 nm). Compared to AgBr/Ag, Ag3PO4/AgBr heterocrystals and pure Ag3PO4 crystals, the heterostructured Ag3PO4/AgBr/Ag plasmonic photocatalysts exhibit much higher photocatalytic activity and stability. This enhanced photocatalytic activity suggests that the synergetic effects of the heterostructured Ag3PO4/AgBr/Ag and the strong SPR of Ag NPs on the surface result in the high efficiencies of the photocatalytic activity and the improved stability. With the assistance of Ag3PO4/AgBr/Ag heterostructures, only 8 min and 12 min are taken to completely decompose MO and MB molecules under visible-light irradiation, respectively. Furthermore, the photodegradation rate does not show an obvious decrease during ten successive cycles, indicating that our heterostructured Ag3PO4/AgBr/Ag plasmonic photocatalysts are extremely stable under visible-light irradiation.
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Cites
Liu, J., Bai, H., Wang, Y., Liu, Z., Zhang, X., & Sun, D. D. (2010) · Advanced Functional Materials · doi:10.1002/adfm.201001391 · Cited by 776
Cited by
Zhang, S., Li, J., Wang, X., Huang, Y., Zeng, M., & Xu, J. (2014) · ACS Applied Materials & Interfaces · doi:10.1021/am505528c · Cited by 432
Yao, X., Liu, X., & Hu, X. (2014) · ChemCatChem · doi:10.1002/cctc.201402487 · Cited by 64
Metadata
- Authors
- Wang, W.-S., Du, H., Wang, R.-X., Wen, T., & Xu, A.-W.
- Venue
- Nanoscale
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2013
- Volume
- 5
- Issue
- 8
- Pages
- 3315
- ISSN
- 2040-3364 (ISSN-L)
- 2040-3372
- OpenAlex
- W2004160113
- Cited by
- 177
- References
- 1
- FWCI
- 8.54
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, W.-S., Du, H., Wang, R.-X., Wen, T., & Xu, A.-W. (2013). Heterostructured Ag3PO4/AgBr/Ag plasmonic photocatalyst with enhanced photocatalytic activity and stability under visible light. Nanoscale. https://doi.org/10.1039/c3nr00191a
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