The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
A hydrazone-based covalent organic framework for photocatalytic hydrogen production
Open accessAbstract
Covalent organic frameworks (COFs) have recently emerged as a new generation of porous polymers combining molecular functionality with the robustness and structural definition of crystalline solids. Drawing on the recent development of tailor-made semiconducting COFs, we report here on a new COF capable of visible-light driven hydrogen generation in the presence of Pt as a proton reduction catalyst (PRC). The COF is based on hydrazone-linked functionalized triazine and phenyl building blocks and adopts a layered structure with a honeycomb-type lattice featuring mesopores of 3.8 nm and the highest surface area among all hydrazone-based COFs reported to date. When illuminated with visible light, the Pt-doped COF continuously produces hydrogen from water without signs of degradation. With their precise molecular organization and modular structure combined with high porosity, photoactive COFs represent well-defined model systems to study and adjust the molecular entities central to the photocatalytic process.
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Semiconductor-based Photocatalytic Hydrogen Generation
Chen, X., Shen, S., Guo, L., & Mao, S. S. (2010) · Chemical Reviews · doi:10.1021/cr1001645 · Cited by 7,876
Cited by
Sulfone-containing covalent organic frameworks for photocatalytic hydrogen evolution from water
Wang, X., Chen, L., Chong, S. Y., Little, M. A., Wu, Y., Zhu, W.-H., Clowes, R., Yan, Y., Zwijnenburg, M. A., Sprick, R. S., et al. (2018) · Nature Chemistry · doi:10.1038/s41557-018-0141-5 · Cited by 1,320
Covalent Organic Framework Photocatalysts: Structures and Applications
Wang, H., Wang, H., Wang, Z., Tang, L., Zeng, G., Xu, P., Chen, M., Xiong, T., Zhou, C., Li, X., et al. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00278j · Cited by 1,301
Liu, R., Tan, K. T., Gong, Y., Chen, Y., Li, Z., Xie, S., He, T., Lu, Z., Yang, H., & Jiang, D. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00620c · Cited by 1,083
Wang, H., Zeng, Z., Xu, P., Li, L., Zeng, G., Xiao, R., Tang, Z., Huang, D., Tang, L., Lai, C., et al. (2019) · Chemical Society Reviews · doi:10.1039/c8cs00376a · Cited by 804
Interface-Assisted Synthesis of 2D Materials: Trend and Challenges
Dong, R., Zhang, T., & Feng, X. (2018) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00056 · Cited by 710
Metadata
- Authors
- Stegbauer, L., Schwinghammer, K., & Lotsch, B. V.
- Venue
- Chem. Sci.
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2014-03-17
- Volume
- 5
- Issue
- 7
- Pages
- 2789-2793
- ISSN
- 2041-6520 (ISSN-L)
- 2041-6539
- OpenAlex
- W1971865766
- Cited by
- 1,145
- References
- 1
- FWCI
- 23.23
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Stegbauer, L., Schwinghammer, K., & Lotsch, B. V. (2014). A hydrazone-based covalent organic framework for photocatalytic hydrogen production. Chem. Sci. https://doi.org/10.1039/c4sc00016a
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