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The effect of the pore-wall structure of carbon nitride on photocatalytic CO2reduction under visible light
Open accessAbstract
Carbon nitride (C3N4) polymers work as a vital component in a photocatalytic CO2 reduction assembly that operates under visible light when modified with a ruthenium complex, trans(Cl)-[Ru{4,4′-(CH2PO3H2)2-2,2′-bipyridine}(CO)2Cl2], (Ru) as a catalyst. Here we examined the effects of structural properties of carbon nitride on the photocatalytic performance for CO2 reduction into formic acid. Introduction of mesoporosity into the graphitic carbon nitride structure increased the specific surface area, leading to significant enhancement in activity. However, higher surface area (in other words, lower crystallinity) that originated from excessively introduced mesopores had a negative impact on activity, although it is a prerequisite to allow for adsorption of Ru on the carbon nitride surface. Thus, the activity was sensitive to specific surface area and crystallinity of carbon nitride, but is largely insensitive to the pore size and the volume.
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Cited by
Ong, W.-J., Tan, L.-L., Ng, Y. H., Yong, S.-T., & Chai, S.-P. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00075 · Cited by 7,147
Cocatalysts for Selective Photoreduction of CO2into Solar Fuels
Li, X., Yu, J., Jaroniec, M., & Chen, X. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00400 · Cited by 2,304
Ran, J., Jaroniec, M., & Qiao, S. (2018) · Advanced Materials · doi:10.1002/adma.201704649 · Cited by 1,531
Recent Advances in Heterogeneous Photocatalytic CO 2 Conversion to Solar Fuels
Li, K., Peng, B., & Peng, T. (2016) · ACS Catalysis · doi:10.1021/acscatal.6b02089 · Cited by 1,355
Insight on Reaction Pathways of Photocatalytic CO2 Conversion
Wang, Y., Chen, E., & Tang, J. (2022) · ACS Catalysis · doi:10.1021/acscatal.2c01012 · Cited by 566
Metadata
- Authors
- Maeda, K., Kuriki, R., Zhang, M., Wang, X., & Ishitani, O.
- Venue
- J. Mater. Chem. A
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2014-07-21
- Volume
- 2
- Issue
- 36
- Pages
- 15146-15151
- ISSN
- 2050-7488 (ISSN-L)
- 2050-7496
- OpenAlex
- W2036104331
- Cited by
- 212
- References
- 0
- FWCI
- 8.84
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- CoChat. (2026). Citation check: The effect of the pore-wall structure of carbon nitride on photocatalytic CO2reduction under visible light. https://app.cochat.ai/papers/10.1039/c4ta03128h
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- Maeda, K., Kuriki, R., Zhang, M., Wang, X., & Ishitani, O. (2014). The effect of the pore-wall structure of carbon nitride on photocatalytic CO2reduction under visible light. J. Mater. Chem. A. https://doi.org/10.1039/c4ta03128h
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