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Ultra-stretchable graphene aerogels at ultralow temperatures
Abstract
Graphene aerogels (GAs) possess workable deformation and sensing properties at extreme temperatures. However, their poor tensile properties have restricted their applications in stretchable electronic devices, smart soft robots, and aerospace. Herein, an ultra-stretchable and elastic graphene aerogel with record elongation from -95% to 400% was achieved by constructing a highly crimped and crosslinked graphene network using a microbubble-filled GA precursor by a simple compress-annealing process. This conductive aerogel with near zero Poisson's ratio showed rubber-like but temperature-invariant elasticity from 196.5 °C to 300 °C, and special strain insensitivity from 50% to 400% tensile strain and high sensitivity below 50% tensile strain. Therefore, it can be used as a highly stretchable but strain-insensitive conductor under extreme environments, in which these polymer-based stretchable conductive materials are not workable. Moreover, this work provides new thoughts on constructing inorganic ultra-stretchable materials.
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“GA is an ideal substrate for constructing monodisperse Pt-based catalysts due to its interconnected 3D network structure and abundant surface defects [16–18].”
From Synergistic interaction of monodisperse Pt nanoparticles with defect‐rich graphene aerogel for efficient acidic hydrogen evolution (2025) · cites this paper as [17]
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Metadata
- Authors
- Yang, G., Zhang, X., Wang, R., Liu, X., Zhang, J., Zong, L., & Yang, H.
- Affiliations
- Qingdao University of Science and Technology (CN)
- Corresponding author
- Zong, Lu
- Yang, Hongsheng
- Venue
- Materials Horizons
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2023
- Volume
- 10
- Issue
- 5
- Pages
- 1865-1874
- ISSN
- 2051-6347 (ISSN-L)
- 2051-6355
- OpenAlex
- W4322485694
- Cited by
- 43
- References
- 40
- Citations by year
- 2026: 6 · 2025: 15 · 2024: 16 · 2023: 6
- FWCI
- 3.40
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Materials Horizons (publishedVersion)
- PubMed (publishedVersion)
- Funders
- Natural Science Foundation of Shandong Province (ZR2022QB022)
- National Natural Science Foundation of China (52202039, 51903134)
- Topics
- Physical Sciences › Engineering › Biomedical Engineering › Advanced Sensor and Energy Harvesting Materials
- Physical Sciences › Materials Science › Materials Chemistry › Graphene research and applications
- Physical Sciences › Materials Science › Materials Chemistry › Aerogels and thermal insulation
- Keywords
- graphene aerogel, high-temperature elasticity, strain insensitivity, Poisson's ratio, stretchable conductors
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