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Dynamics of concentrated polymer systems. Part 4.—Rheological properties
Abstract
The constitutive equation for polymer melts and concentrated solutions derived in the previous papers is applied to two typical rheometrical flows: steady and transient shear flow, oscillatory shear flow superposed on steady flow, steady and transient uniaxial elongational flow. The stress responses predicted are qualitatively in good agreement with experiments except for one case (the first normal stress in the transient shear flow). A particularly interesting result is that the constitutive equation suggests instability in steady shear flow and uniaxial elongational flow.
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Citations
Cited by
Dynamics of entangled linear polymer melts: A molecular-dynamics simulation
Kremer, K., & Grest, G. S. (1990) · The Journal of Chemical Physics · doi:10.1063/1.458541 · Cited by 4,023
Viscoelasticity and dynamics of entangled polymers
Watanabe, H. (1999) · Progress in Polymer Science · doi:10.1016/s0079-6700(99)00029-5 · Cited by 718
Entangled linear, branched and network polymer systems — Molecular theories
Graessley, W. W. (2006) · Advances in Polymer Science · doi:10.1007/bfb0038532 · Cited by 621
The effect of entanglements in rubber elasticity
Edwards, S. F., & Vilgis, T. (1986) · Polymer · doi:10.1016/0032-3861(86)90231-4 · Cited by 460
Self-citationDynamics of entanglements: A nonlinear model consistent with the Cox-Merz rule
Marrucci, G. (1996) · Journal of Non-Newtonian Fluid Mechanics · doi:10.1016/0377-0257(95)01407-1 · Cited by 458
Metadata
- Authors
- Doi, M., & Edwards, S. F.
- Venue
- J. Chem. Soc., Faraday Trans. 2
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 1979
- Volume
- 75
- Issue
- 0
- Pages
- 38-54
- ISSN
- 0300-9238 (ISSN-L)
- OpenAlex
- W2036809892
- Cited by
- 516
- References
- 0
- FWCI
- 16.15
- Type
- journal article
- Language
- en
- Open access
- closed
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