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Re-evaluation of the thiocyanate dosimeter for pulse radiolysis
Abstract
The thiocyanate dosimeter (10–2 mol dm–3 SCN– in O2-saturated water) has been standardised against the super-Fricke dosimeter (10–2 mol dm–3 FeII in O2-saturated 0.4 mol dm–3 H2SO4) using the hexacyanoferrate(II) dosimeter [5 × 10–3 mol dm–3 Fe(CN)64– in O2-saturated water] as a secondary standard. On the basis that G(FeIII)= 1.67 × 10–6 mol J–1 and εFeIII= 220.4 m2 mol–1 at 304 nm and 25 °C in the super-Fricke dosimeter, we obtain Gε[Fe(CN)63–]=(3.47 ± 0.06)× 10–5 m2 J–1 at 420 nm and Gε(SCN)2˙–=(2.59 ± 0.05)× 10–4 m2 J–1 at 475 nm. These values remain unchanged when the solutions are saturated with air instead of O2 and are doubled in N2O-saturated solution.
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Citations
Cites
Buxton, G. V., Greenstock, C. L., Helman, W. P., & Ross, A. B. (1988) · Journal of Physical and Chemical Reference Data · doi:10.1063/1.555805 · Cited by 12,332
Self-citation
Cited by
An, T., Yang, H., Li, G., Song, W., Cooper, W. J., & Nie, X. (2010) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2009.12.002 · Cited by 649
Das, T. N. (2001) · The Journal of Physical Chemistry A · doi:10.1021/jp011255h · Cited by 259
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Goldstein, S., Czapski, G., Lind, J., & Merényi, G. (2000) · Journal of Biological Chemistry · doi:10.1074/jbc.275.5.3031 · Cited by 177
Pezzella, A., Panzella, L., Crescenzi, O., Napolitano, A., Navaratman, S., Edge, R., Land, E. J., Barone, V., & d'Ischia, M. (2006) · Journal of the American Chemical Society · doi:10.1021/ja0650246 · Cited by 112
Pezzella, A., Panzella, L., Crescenzi, O., Napolitano, A., Navaratnam, S., Edge, R., Land, E. J., Barone, V., & d’Ischia, M. (2009) · The Journal of Organic Chemistry · doi:10.1021/jo900250v · Cited by 47
Metadata
- Authors
- Buxton, G. V., & Stuart, C. R.
- Venue
- Journal of the Chemical Society, Faraday Transactions
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 1995
- Volume
- 91
- Issue
- 2
- Pages
- 279
- ISSN
- 0956-5000 (ISSN-L)
- 1364-5455
- OpenAlex
- W2068119928
- Cited by
- 496
- References
- 1
- FWCI
- 23.79
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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