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Acyl Radical Chemistry via Visible-Light Photoredox Catalysis
Open accessAbstract
Visible-light photoredox catalysis enables easy access to acyl radicals under mild reaction conditions. Reactive acyl radicals, generated from various acyl precursors such as aldehydes, α-keto acids, carboxylic acids, anhydrides, acyl thioesters, acyl chlorides, or acyl silanes, can undergo a diverse range of synthetically useful transformations, which were previously difficult or inaccessible. This review summarizes the recent progress on visible-light-driven acyl radical generation using transition-metal photoredox catalysts, metallaphotocatalysts, hypervalent iodine catalysts or organic photocatalysts. 1 Introduction 2 The Scope of This Review 3 Aldehydes as a Source of Acyl Radicals 4 α-Keto Acids as a Source of Acyl Radicals 5 Carboxylic Acids as a Source of Acyl Radicals 6 Anhydrides as a Source of Acyl Radicals 7 Acyl Thioesters as a Source of Acyl Radicals 8 Acyl Chlorides as a Source of Acyl Radicals 9 Acyl Silanes as a Source of Acyl Radicals 10 Conclusions and Future Outlook
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Cites
Prier, C. K., Rankic, D. A., & MacMillan, D. W. C. (2013) · Chemical Reviews · doi:10.1021/cr300503r · Cited by 9,590
Cited by
Liu, K., Schwenzer, M., & Studer, A. (2022) · ACS Catalysis · doi:10.1021/acscatal.2c03996 · Cited by 325
Desulfonylation via Radical Process: Recent Developments in Organic Synthesis
Chu, X.-Q., Ge, D., Cui, Y.-Y., Shen, Z.-L., & Li, C.-J. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.1c00084 · Cited by 259
Metadata
- Authors
- Ngai, M.-Y., Banerjee, A., & Lei, Z.
- Venue
- Synthesis
- Publisher
- Georg Thieme Verlag KG
- Published
- 2018-12-12
- Volume
- 51
- Issue
- 02
- Pages
- 303-333
- ISSN
- 0039-7881 (ISSN-L)
- 1437-210X
- OpenAlex
- W2904940349
- Cited by
- 255
- References
- 1
- FWCI
- 9.77
- Type
- journal article
- Language
- en
- Open access
- green
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- Ngai, M.-Y., Banerjee, A., & Lei, Z. (2019). Acyl Radical Chemistry via Visible-Light Photoredox Catalysis. Synthesis. https://doi.org/10.1055/s-0037-1610329
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