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Equilibrium behavior of asymmetric ABA triblock copolymer melts
Abstract
Melts of ABA triblock copolymers with two different sized end blocks are examined using self-consistent field theory. At small asymmetries, the A block bidispersity reduces the stretching energy of the A domains. This effect causes a slight increase in the domain spacing and shifts the order–order transitions (OOTs) toward higher A volume fractions. At large asymmetries, a significant number of the short A blocks pull free of their domains allowing their B blocks to relax. This effect produces a much greater increase in domain spacing and shifts the OOTs toward lower A volume fractions. It also leads to a sizable region of close-packed spheres. At the crossover between these two effects, the ordered morphologies are shifted from their normal compositions by about 10%. The displacement of the complex gyroid region is found to have a strong influence on the metastability of the perforated-lamellar phase.
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Citations
Cites
Origins of complex self-assembly in block copolymers
Matsen, M. W., & Bates, F. S. (1996) · Macromolecules · doi:10.1021/ma960744q · Cited by 578
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Cited by
Nanostructure fabrication using block copolymers
Hamley, I. W. (2003) · Nanotechnology · doi:10.1088/0957-4484/14/10/201 · Cited by 773
Phase Behaviour and Morphologies of Block Copolymers
Abetz, V., & Simon, P. F. W. (2005) · Advances in Polymer Science · doi:10.1007/12_004 · Cited by 361
Metadata
- Authors
- Matsen, M. W.
- Venue
- The Journal of Chemical Physics
- Publisher
- AIP Publishing
- Published
- 2000-10-01
- Volume
- 113
- Issue
- 13
- Pages
- 5539-5544
- ISSN
- 0021-9606 (ISSN-L)
- 1089-7690
- OpenAlex
- W4230792165
- Cited by
- 181
- References
- 1
- FWCI
- 1.98
- Type
- journal article
- Language
- en
- Open access
- closed
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