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Structures of small gold cluster cations (Aun+, n<14): Ion mobility measurements versus density functional calculations
Abstract
We have performed ion mobility measurements on gold cluster cations Aun+ generated by pulsed laser vaporization. For clusters with n<14, experimental cross sections are compared with theoretical results from density functional calculations. This comparison allows structural assignment. We find that room temperature gold cluster cations have planar structures for n=3–7. Starting at n=8 they form three dimensional structures with (slightly distorted) fragments of the bulk phase structure being observed for n=8–10.
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Cited by
Structural properties of nanoclusters: Energetic, thermodynamic, and kinetic effects
Baletto, F., & Ferrando, R. (2005) · Reviews of Modern Physics · doi:10.1103/revmodphys.77.371 · Cited by 1,811
Häkkinen, H., Yoon, B., Landman, U., Li, X., Zhai, H.-J., & Wang, L.-S. (2003) · The Journal of Physical Chemistry A · doi:10.1021/jp035437i · Cited by 631
Recommendations for reporting ion mobility Mass Spectrometry measurements
Gabelica, V., Shvartsburg, A. A., Afonso, C., Barran, P., Benesch, J. L. P., Bleiholder, C., Bowers, M. T., Bilbao, A., Bush, M. F., Campbell, J. L., et al. (2019) · Mass Spectrometry Reviews · doi:10.1002/mas.21585 · Cited by 493
2D-3D transition of gold cluster anions resolved
Johansson, M. P., Lechtken, A., Schooss, D., Kappes, M. M., & Furche, F. (2008) · Physical Review A · doi:10.1103/physreva.77.053202 · Cited by 273
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Metadata
- Authors
- Gilb, S., Weis, P., Furche, F., Ahlrichs, R., & Kappes, M. M.
- Venue
- The Journal of Chemical Physics
- Publisher
- AIP Publishing
- Published
- 2002-03-08
- Volume
- 116
- Issue
- 10
- Pages
- 4094-4101
- ISSN
- 0021-9606 (ISSN-L)
- 1089-7690
- OpenAlex
- W1584114617
- Cited by
- 462
- References
- 0
- FWCI
- 15.21
- Type
- journal article
- Language
- en
- Open access
- closed
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- Gilb, S., Weis, P., Furche, F., Ahlrichs, R., & Kappes, M. M. (2002). Structures of small gold cluster cations (Aun+, n<14): Ion mobility measurements versus density functional calculations. The Journal of Chemical Physics. https://doi.org/10.1063/1.1445121
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