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Theory of the Interface between Immiscible Polymers. II
Abstract
A theory is developed to predict the interfacial properties between two immiscible polymers. A self-consistent-field approach is employed to describe the configurational statistics of polymer molecules in the interfacial region. The density profiles and surface tension are calculated, and compare well with experiments. The interfaces are found to be much broader than for ordinary liquids. Also discussed are the distribution of chain ends and block-copolymer joints in the interface, and the effects of adding moderate amounts of solvent.
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Citations
Cited by
Block Copolymers: Past Successes and Future Challenges
Lodge, T. P. (2003) · Macromolecular Chemistry and Physics · doi:10.1002/macp.200290073 · Cited by 567
Biological and synthetic membranes: What can be learned from a coarse-grained description?
MULLER, M., KATSOV, K., & SCHICK, M. (2006) · Physics Reports · doi:10.1016/j.physrep.2006.08.003 · Cited by 320
Molecular aspects of muco- and bioadhesion:
Huang, Y., Leobandung, W., Foss, A., & Peppas, N. A. (2000) · Journal of Controlled Release · doi:10.1016/s0168-3659(99)00233-3 · Cited by 316
Daoulas, K. C., Theodorou, D. N., Roos, A., & Creton, C. (2004) · Macromolecules · doi:10.1021/ma035383a · Cited by 41
Metadata
- Authors
- Helfand, E., & Tagami, Y.
- Venue
- The Journal of Chemical Physics
- Publisher
- AIP Publishing
- Published
- 1972-04-01
- Volume
- 56
- Issue
- 7
- Pages
- 3592-3601
- ISSN
- 0021-9606 (ISSN-L)
- 1089-7690
- OpenAlex
- W1999865376
- Cited by
- 1,009
- References
- 0
- FWCI
- 3.82
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Theory of the Interface between Immiscible Polymers. II. https://app.cochat.ai/papers/10.1063/1.1677735
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- Helfand, E., & Tagami, Y. (1972). Theory of the Interface between Immiscible Polymers. II. The Journal of Chemical Physics. https://doi.org/10.1063/1.1677735
Data sources
Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
