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Absolute Intensities of the Discrete and Continuous Absorption Bands of Oxygen Gas at 1.26 and 1.065 μ and the Radiative Lifetime of the 1Δ g State of Oxygen
Open accessAbstract
Laboratory measurements have been made of the absolute intensities of the discrete-line absorption band at 1.26 μ, and of the continuous bands at 1.26 and 1.065 μ in oxygen gas at pressures up to 4.3 atm. It has been shown that discrete and continuous absorptions are quite independent features, the one being a measure of the intrinsic transition probability in isolated molecules, the other of its enhancement in collision complexes. In the former the lines show significant pressure broadening, but the integral molecular absorption coefficients are constant; in the latter they are proportional to pressure and continuous absorption dominates in the 1.26-μ region at about ½ atm oxygen pressure. The radiative half-life of isolated 1Δg oxygen molecules is estimated to be 45 min, and the effect of gas pressure on the rate of decay has been predicted.
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Cites
Kombinationsbeziehungen im Absorptionsspektrum des fl�ssigen Sauerstoffs
Ellis, J. W., & Kneser, H. O. (1933) · The European Physical Journal A · doi:10.1007/bf01338969 · Cited by 103
Cited by
Physical Mechanisms of Generation and Deactivation of Singlet Oxygen
Schweitzer, C., & Schmidt, R. (2003) · Chemical Reviews · doi:10.1021/cr010371d · Cited by 2,123
THE HITRAN MOLECULAR SPECTROSCOPIC DATABASE AND HAWKS (HITRAN ATMOSPHERIC WORKSTATION): 1996 EDITION
ROTHMAN, L. S., RINSLAND, C. P., GOLDMAN, A., MASSIE, S. T., EDWARDS, D. P., FLAUD, J.-M., PERRIN, A., CAMY-PEYRET, C., DANA, V., MANDIN, J.-Y., et al. (1998) · Journal of Quantitative Spectroscopy and Radiative Transfer · doi:10.1016/s0022-4073(98)00078-8 · Cited by 1,925
AFGL atmospheric absorption line parameters compilation: 1982 edition
Rothman, L. S., Gamache, R. R., Barbe, A., Goldman, A., Gillis, J. R., Brown, L. R., Toth, R. A., Flaud, J.-M., & Camy-Peyret, C. (1983) · Applied Optics · doi:10.1364/ao.22.002247 · Cited by 447
Physics and engineering of singlet delta oxygen production in low-temperature plasma
Ionin, A. A., Kochetov, I. V., Napartovich, A. P., & Yuryshev, N. N. (2007) · Journal of Physics D: Applied Physics · doi:10.1088/0022-3727/40/2/r01 · Cited by 292
Metadata
- Authors
- Badger, R. M., Wright, A. C., & Whitlock, R. F.
- Venue
- The Journal of Chemical Physics
- Publisher
- AIP Publishing
- Published
- 1965-12-15
- Volume
- 43
- Issue
- 12
- Pages
- 4345-4350
- ISSN
- 0021-9606 (ISSN-L)
- 1089-7690
- OpenAlex
- W2036734647
- Cited by
- 329
- References
- 1
- FWCI
- 6.97
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Badger, R. M., Wright, A. C., & Whitlock, R. F. (1965). Absolute Intensities of the Discrete and Continuous Absorption Bands of Oxygen Gas at 1.26 and 1.065 μ and the Radiative Lifetime of the 1Δ g State of Oxygen. The Journal of Chemical Physics. https://doi.org/10.1063/1.1696694
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