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Influence of Energy Transfer by the Exchange Mechanism on Donor Luminescence
Abstract
The decay of donor luminescence in a rigid solution when modified by electronic energy transfer by the exchange mechanism is treated theoretically. The rate constant for the elementary process of energy transfer is taken to be of the Dexter form, const exp(−2R/L), where R is the donor—acceptor distance and L is a positive constant. Calculations are made of the yield and decay time of the donor luminescence as functions of the acceptor concentration. The resulting relationship among the above quantities enables one to analyze experimental data in a quantitative manner, and thereby to obtain information about an intermolecular exchange interaction. As an example of such an analysis, Ermolaev's data on triplet—triplet transfer between some aromatic molecules are compared with our results, and very good agreement is found with a choice of the single parameter L.
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Citations
Cited by
Winkler, J. R., & Gray, H. B. (2014) · Journal of the American Chemical Society · doi:10.1021/ja500215j · Cited by 306
Chemically Produced Excited States
White, E. H., Miano, J. D., Watkins, C. J., & Breaux, E. J. (1974) · Angewandte Chemie International Edition in English · doi:10.1002/anie.197402291 · Cited by 99
Metadata
- Authors
- Inokuti, M., & Hirayama, F.
- Venue
- The Journal of Chemical Physics
- Publisher
- AIP Publishing
- Published
- 1965-09-15
- Volume
- 43
- Issue
- 6
- Pages
- 1978-1989
- ISSN
- 0021-9606 (ISSN-L)
- 1089-7690
- OpenAlex
- W2033633102
- Cited by
- 2,468
- References
- 0
- FWCI
- 6.75
- Type
- journal article
- Language
- en
- Open access
- closed
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- Inokuti, M., & Hirayama, F. (1965). Influence of Energy Transfer by the Exchange Mechanism on Donor Luminescence. The Journal of Chemical Physics. https://doi.org/10.1063/1.1697063
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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