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Raman Spectral Studies of Water Structure
Abstract
Raman frequencies and polarizations and infrared frequencies of water and heavy water have been obtained, and the intermolecular vibrations of water have been related to a five-molecule hydrogen-bonded C2v model consistent with x-ray data. Observed variations of the integrated Raman intensity of the 175-cm—1 hydrogen-bond-stretching vibration, with variations of temperature, have been interpreted in terms of the five-molecule model. That interpretation leads to reasonable values for the enthalpy of hydrogen-bond formation. Effects of electrolyte addition on the intensity of the 175-cm—1 band are also described.
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“We found that the double donor-double acceptor (DDAA) centered at 3226 cm 1 and the single donor-single acceptor (DA) centered at 3432 cm 1 , which have tetrahedral structure and chains structure of water, respectively [65,66], were consistently the dominant types in the four solutions.”
From Effect of Hofmeister Anions on Interfacial Properties of Mica Surface in Concentrated Aqueous Solution (2020) · cites this paper as [66]
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Research works printed but not linked: 24
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Kan, Y., Yang, Q., Zhang, X., & Zhang, Y. (2020) · Coatings · doi:10.3390/coatings10090872 · Cited by 4
“We found that the double donor-double acceptor (DDAA) centered at 3226 cm−1 and the single donor-single acceptor (DA) centered at 3432 cm−1, which have tetrahedral structure and chains structure of water, respectively [65,66], were consistently the dominant types in the four solutions.”
Background
Metadata
- Authors
- Walrafen, G. E.
- Affiliations
- Bell Telephone Laboratories, Inc., Murray Hill, New Jersey
- Corresponding author
- Walrafen, G. E.
- Venue
- The Journal of Chemical Physics
- Publisher
- AIP Publishing
- Published
- 1964-06-01
- Volume
- 40
- Issue
- 11
- Pages
- 3249-3256
- ISSN
- 0021-9606 (ISSN-L)
- 1089-7690
- OpenAlex
- W1979193828
- Cited by
- 629
- References
- 0
- Citations by year
- 2026: 17 · 2025: 22 · 2024: 17 · 2023: 17 · 2022: 13 · 2021: 21 · 2020: 24 · 2019: 23 · 2018: 21 · 2017: 13 · 2016: 21 · 2015: 25 · 2014: 19 · 2013: 15 · 2012: 17
- FWCI
- 6.54
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- The Journal of Chemical Physics (publishedVersion)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Spectroscopy and Quantum Chemical Studies
- Physical Sciences › Chemistry › Spectroscopy › Molecular Spectroscopy and Structure
- Life Sciences › Biochemistry, Genetics and Molecular Biology › Biophysics › Spectroscopy Techniques in Biomedical and Chemical Research
- Keywords
- water structure, heavy water, intermolecular vibrations, hydrogen-bonded clusters, Raman intensity, infrared frequencies, temperature dependence, electrolyte effects
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