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Hollow nanostructures based on the Kirkendall effect: Design and stability considerations
Abstract
In nanoscale interdiffusion and reaction, a Kirkendall void in the core of a nanocrystal has been proposed to explain the formation of hollow nanosize particles in recent literature. We present here a simple kinetic analysis of the reaction in nanoparticles, including the effect of the Gibbs–Thomson potential. A general discussion on how to form hollow nanostructures utilizing the mechanism of the Kirkendall effect is given. Furthermore, we show that a hollow nanosize particle is thermodynamically unstable; a high-temperature aging will drive thermal vacancies to the outer surface and transform the hollow nanocrystal to a solid nanocrystal.
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Cites
A Rational Theory of the Size of Government
Meltzer, A. H., & Richard, S. F. (1981) · Journal of Political Economy · doi:10.1086/261013 · Cited by 5,485
The Penn World Table (Mark 5): An Expanded Set of International Comparisons, 1950-1988
Summers, R., & Heston, A. (1991) · The Quarterly Journal of Economics · doi:10.2307/2937941 · Cited by 3,429
Cited by
Fan, H. J., Gösele, U., & Zacharias, M. (2007) · Small · doi:10.1002/smll.200700382 · Cited by 962
Self-citationSynthetic architecture of interior space for inorganic nanostructures
Zeng, H. C. (2006) · J. Mater. Chem. · doi:10.1039/b511296f · Cited by 462
Fan, H. J., Knez, M., Scholz, R., Hesse, D., Nielsch, K., Zacharias, M., & Gösele, U. (2007) · Nano Letters · doi:10.1021/nl070026p · Cited by 401
Self-citationZheng, Y., Shang, P., Pei, F., Ma, G., Ye, Z., Peng, X., & Li, D. (2022) · Chemical Engineering Journal · doi:10.1016/j.cej.2022.134571 · Cited by 40
Metadata
- Authors
- Tu, K. N., & Gösele, U.
- Venue
- Applied Physics Letters
- Publisher
- AIP Publishing
- Published
- 2005-02-25
- Volume
- 86
- Issue
- 9
- ISSN
- 0003-6951 (ISSN-L)
- 1077-3118
- OpenAlex
- W2013269378
- Cited by
- 238
- References
- 2
- FWCI
- 7.46
- Type
- journal article
- Language
- en
- Open access
- closed
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