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On the orientational relaxation of HDO in liquid water
Abstract
We use femtosecond mid-infrared pump-probe spectroscopy to study the orientational relaxation of HDO molecules dissolved in H2O. In order to obtain a reliable anisotropy decay we model the effects of heating and correct for these effects. We have measured the reorientation time constant of the OD vibration from 2430to2600cm−1, and observe a value of 2.5ps that shows no variation over this frequency interval. Our results are discussed in the context of previous experiments that have been performed on the complementary system of HDO dissolved in D2O.
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Citations
Cited by
On the Molecular Mechanism of Water Reorientation
Laage, D., & Hynes, J. T. (2008) · The Journal of Physical Chemistry B · doi:10.1021/jp805217u · Cited by 438
Medders, G. R., Babin, V., & Paesani, F. (2014) · Journal of Chemical Theory and Computation · doi:10.1021/ct5004115 · Cited by 435
The Properties of Water: Insights from Quantum Simulations
Paesani, F., & Voth, G. A. (2009) · The Journal of Physical Chemistry B · doi:10.1021/jp810590c · Cited by 256
Time-Resolved Studies of Water Dynamics and Proton Transfer at the Alumina−Air Interface
Le Caër, S., Palmer, D. J., Lima, M., Renault, J. P., Vigneron, G., Righini, R., & Pommeret, S. (2007) · Journal of the American Chemical Society · doi:10.1021/ja0691730 · Cited by 25
Metadata
- Authors
- Rezus, Y. L. A., & Bakker, H. J.
- Venue
- The Journal of Chemical Physics
- Publisher
- AIP Publishing
- Published
- 2005-09-15
- Volume
- 123
- Issue
- 11
- Pages
- 114502-114502
- ISSN
- 0021-9606 (ISSN-L)
- 1089-7690
- OpenAlex
- W2064141166
- Cited by
- 258
- References
- 0
- FWCI
- 8.20
- Type
- journal article
- Language
- en
- Open access
- closed
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- Rezus, Y. L. A., & Bakker, H. J. (2005). On the orientational relaxation of HDO in liquid water. The Journal of Chemical Physics. https://doi.org/10.1063/1.2009729
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