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Surface selection rules
Abstract
The modification of the absorption, emission, and Raman scattering intensities of molecules near metal surfaces is discussed with emphasis on the last. These modifications are usually referred to as surface selection rules. We show that in Raman scattering, the ‘‘rule,’’ which states that only those modes will be active which belong to the irreducible representation to which α′zz also belongs, is only approximately obeyed. The circumstances under which modes which are represented by nondiagonal derived polarizibility tensors are ‘‘surface-active’’ are considered, as well as the geometrical strategies which should be followed in studying the Raman spectra of molecules adsorbed on flat, metal surfaces.
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Cites
Optical Constants of the Noble Metals
Johnson, P. B., & Christy, R. W. (1972) · Physical Review B · doi:10.1103/physrevb.6.4370 · Cited by 20,094
Cited by
Fundamental understanding and applications of plasmon-enhanced Raman spectroscopy
Wang, X., Huang, S.-C., Hu, S., Yan, S., & Ren, B. (2020) · Nature Reviews Physics · doi:10.1038/s42254-020-0171-y · Cited by 689
Guerrini, L., & Graham, D. (2012) · Chemical Society Reviews · doi:10.1039/c2cs35118h · Cited by 441
Raman spectra of size-selected silicon clusters and comparison with calculated structures
Honea, E. C., Ogura, A., Murray, C. A., Raghavachari, K., Sprenger, W. O., Jarrold, M. F., & Brown, W. L. (1993) · Nature · doi:10.1038/366042a0 · Cited by 391
(2025) · doi:10.1021/acschembio.4c00576 · Cited by 12
Metadata
- Authors
- Moskovits, M.
- Venue
- The Journal of Chemical Physics
- Publisher
- AIP Publishing
- Published
- 1982-11-01
- Volume
- 77
- Issue
- 9
- Pages
- 4408-4416
- ISSN
- 0021-9606 (ISSN-L)
- 1089-7690
- OpenAlex
- W2024236859
- Cited by
- 707
- References
- 1
- FWCI
- 5.04
- Type
- journal article
- Language
- en
- Open access
- closed
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