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Experimental observation of the negatively charged water dimer and other small (H2O)−n clusters
Abstract
Beams of (H2O)−n and (D2O)−n have been produced by injecting low energy electrons into a supersonic expansion of water and heavy water seeded in rare gases. Clusters with n≥2, with the exception of n=4, have been observed. The size distribution can be separated into three groups (n=2, n=6–7, and n≥10), which may be associated with different types of electron binding. The n<10 result gives a new lower limit for the number of water molecules necessary to bind an electron; the n≥10 correspond to the n=11 threshold observed earlier in pure H2O expansions.
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Cited by
Noncovalent interactions: A challenge for experiment and theory
Müller-Dethlefs, K., & Hobza, P. (2000) · Chemical Reviews · doi:10.1021/cr9900331 · Cited by 1,781
Gregory, J. K., & Clary, D. C. (1996) · The Journal of Physical Chemistry · doi:10.1021/jp9616019 · Cited by 261
Metadata
- Authors
- Haberland, H., Ludewigt, C., Schindler, H.-G., & Worsnop, D. R.
- Venue
- The Journal of Chemical Physics
- Publisher
- AIP Publishing
- Published
- 1984-10-15
- Volume
- 81
- Issue
- 8
- Pages
- 3742-3744
- ISSN
- 0021-9606 (ISSN-L)
- 1089-7690
- OpenAlex
- W2069087497
- Cited by
- 236
- References
- 0
- FWCI
- 5.53
- Type
- journal article
- Language
- en
- Open access
- closed
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- Haberland, H., Ludewigt, C., Schindler, H.-G., & Worsnop, D. R. (1984). Experimental observation of the negatively charged water dimer and other small (H2O)−n clusters. The Journal of Chemical Physics. https://doi.org/10.1063/1.448127
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