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Control of selectivity of chemical reaction via control of wave packet evolution
Abstract
A time-dependent formulation of two-photon spectroscopy is employed to show that selectivity of reactivity can be achieved via coherent two-photon processes. The problem of finding the optimum waveform (i.e., coherent pulse sequence) that will maximize the formation of a desired chemical species is formulated as a problem in the calculus of variations, and solved for two different cases.
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Citations
Cited by
Khaneja, N., Reiss, T., Kehlet, C., Schulte-Herbrüggen, T., & Glaser, S. J. (2005) · Journal of Magnetic Resonance · doi:10.1016/j.jmr.2004.11.004 · Cited by 1,854
Nanoplasmonics: Past, present, and glimpse into future
Stockman, M. I. (2011) · Optics Express · doi:10.1364/oe.19.022029 · Cited by 1,109
Laser Control of Chemical Reactions
Zare, R. N. (1998) · Science · doi:10.1126/science.279.5358.1875 · Cited by 580
Quantum mechanical optimal control of physical observables in microsystems
Shi, S., & Rabitz, H. (1990) · The Journal of Chemical Physics · doi:10.1063/1.458438 · Cited by 323
Monotonically convergent optimization in quantum control using Krotov’s method
Reich, D. M., Ndong, M., & Koch, C. P. (2012) · The Journal of Chemical Physics · doi:10.1063/1.3691827 · Cited by 220
Metadata
- Authors
- Tannor, D. J., & Rice, S. A.
- Venue
- The Journal of Chemical Physics
- Publisher
- AIP Publishing
- Published
- 1985-11-15
- Volume
- 83
- Issue
- 10
- Pages
- 5013-5018
- ISSN
- 0021-9606 (ISSN-L)
- 1089-7690
- OpenAlex
- W2026008088
- Cited by
- 990
- References
- 0
- FWCI
- 4.29
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Control of selectivity of chemical reaction via control of wave packet evolution. https://app.cochat.ai/papers/10.1063/1.449767
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- Tannor, D. J., & Rice, S. A. (1985). Control of selectivity of chemical reaction via control of wave packet evolution. The Journal of Chemical Physics. https://doi.org/10.1063/1.449767
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
