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Noncrystalline structure of argon clusters. II. Multilayer icosahedral structure of Ar N clusters 50<N<750
Abstract
In a preceding paper, we have described the polyicosahedral structure of small argon clusters containing less than about 50 atoms which were produced in a free jet expansion. Going on with this study, we describe presently the multilayer icosahedral structure of larger argon clusters containing up to about 750 atoms, a value for which the transition to the fcc crystalline bulk structure is found to occur. Cluster models are used in order to study the third icosahedral layer construction, and the transition from a twin to a regular surface arrangement, which is expected to take place around 75 atoms, is observed on experimental patterns. The good agreement between experimental and calculated diffraction functions leads to an estimate of mean cluster sizes, cluster size distributions, and temperature (32±2 K) of clusters containing several hundreds of atoms.
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Cited by
Structural properties of nanoclusters: Energetic, thermodynamic, and kinetic effects
Baletto, F., & Ferrando, R. (2005) · Reviews of Modern Physics · doi:10.1103/revmodphys.77.371 · Cited by 1,811
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Ditmire, T., Donnelly, T., Rubenchik, A. M., Falcone, R. W., & Perry, M. D. (1996) · Physical Review A · doi:10.1103/physreva.53.3379 · Cited by 855
The 3D-architecture of individual free silver nanoparticles captured by X-ray scattering
Barke, I., Hartmann, H., Rupp, D., Flückiger, L., Sauppe, M., Adolph, M., Schorb, S., Bostedt, C., Treusch, R., Peltz, C., et al. (2015) · Nature Communications · doi:10.1038/ncomms7187 · Cited by 100
Metadata
- Authors
- Farges, J., de Feraudy, M. F., Raoult, B., & Torchet, G.
- Venue
- The Journal of Chemical Physics
- Publisher
- AIP Publishing
- Published
- 1986-03-15
- Volume
- 84
- Issue
- 6
- Pages
- 3491-3501
- ISSN
- 0021-9606 (ISSN-L)
- 1089-7690
- OpenAlex
- W2085447425
- Cited by
- 471
- References
- 0
- FWCI
- 16.27
- Type
- journal article
- Language
- en
- Open access
- closed
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- Farges, J., de Feraudy, M. F., Raoult, B., & Torchet, G. (1986). Noncrystalline structure of argon clusters. II. Multilayer icosahedral structure of Ar N clusters 50<N<750. The Journal of Chemical Physics. https://doi.org/10.1063/1.450235
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