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Extraction of kinetic parameters in temperature programmed desorption: A comparison of methods
Abstract
An investigation of the temperature programmed desorption (TPD) of CO and D2 from Ni(111) has been carried out. It has been shown that a differential method for the extraction of the kinetic parameters, threshold temperature programmed desorption (TTPD), can be applied with accuracy near the limit of zero coverage. In this limit, agreement is found between integral and differential methods for kinetic parameter evaluation. The factors which limit the applicability of TTPD are explored and a method to verify its proper application is presented.
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Cited by
Wellendorff, J., Silbaugh, T. L., Garcia-Pintos, D., Nørskov, J. K., Bligaard, T., Studt, F., & Campbell, C. T. (2015) · Surface Science · doi:10.1016/j.susc.2015.03.023 · Cited by 572
Campbell, C. T. (1994) · Topics in Catalysis · doi:10.1007/bf01492288 · Cited by 314
Femtomole Adsorption Calorimetry on Single-Crystal Surfaces
Brown, W. A., Kose, R., & King, D. A. (1998) · Chemical Reviews · doi:10.1021/cr9700890 · Cited by 306
Abild-Pedersen, F., & Andersson, M. P. (2007) · Surface Science · doi:10.1016/j.susc.2007.01.052 · Cited by 306
Study of high coverages of atomic oxygen on the Pt(111) surface
Parker, D. H., Bartram, M. E., & Koel, B. E. (1989) · Surface Science · doi:10.1016/0039-6028(89)90443-3 · Cited by 289
Metadata
- Authors
- Miller, J. B., Siddiqui, H. R., Gates, S. M., Russell, J. N., Yates, J. T., Tully, J. C., & Cardillo, M. J.
- Venue
- The Journal of Chemical Physics
- Publisher
- AIP Publishing
- Published
- 1987-12-01
- Volume
- 87
- Issue
- 11
- Pages
- 6725-6732
- ISSN
- 0021-9606 (ISSN-L)
- 1089-7690
- OpenAlex
- W2024651849
- Cited by
- 247
- References
- 0
- FWCI
- 9.75
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Extraction of kinetic parameters in temperature programmed desorption: A comparison of methods. https://app.cochat.ai/papers/10.1063/1.453409
- The paper
- Miller, J. B., Siddiqui, H. R., Gates, S. M., Russell, J. N., Yates, J. T., Tully, J. C., & Cardillo, M. J. (1987). Extraction of kinetic parameters in temperature programmed desorption: A comparison of methods. The Journal of Chemical Physics. https://doi.org/10.1063/1.453409
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
