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Transient solvation of polar dye molecules in polar aprotic solvents
Abstract
Subpicosecond fluorescence spectroscopy of the polar dye molecules coumarin 311 and coumarin 102 has been used to measure the microscopic solvation dynamics of several polar aprotic solvents. The measured solvation times are significantly longer than the longitudinal relaxation times τ1 of the solvents. τ1 is the predicted time for solvation according to dielectric continuum theory. The experiments were made with a newly constructed subpicosecond ultraviolet emission apparatus that takes advantage of recent advances in ultrafast laser technology. The newly developed, time saving procedure [Nagarajan et al., J. Chem. Phys. 86, 3183 (1987)] for measuring the microscopic solvation response functions was used in this research.
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Citations
Cites
Dielectric properties and relaxation in ethylene carbonate and propylene carbonate
Payne, R., & Theodorou, I. E. (1972) · The Journal of Physical Chemistry · doi:10.1021/j100664a019 · Cited by 254
Cited by
The dynamics of solvation in polar liquids
Maroncelli, M. (1993) · Journal of Molecular Liquids · doi:10.1016/0167-7322(93)80045-w · Cited by 719
Computer simulation of the dynamics of aqueous solvation
Maroncelli, M., & Fleming, G. R. (1988) · The Journal of Chemical Physics · doi:10.1063/1.455649 · Cited by 494
Water Immobilization at Surfactant Interfaces in Reverse Micelles
Riter, R. E., Willard, D. M., & Levinger, N. E. (1998) · The Journal of Physical Chemistry B · doi:10.1021/jp973330n · Cited by 290
Metadata
- Authors
- Kahlow, M. A., Kang, T. J., & Barbara, P. F.
- Venue
- The Journal of Chemical Physics
- Publisher
- AIP Publishing
- Published
- 1988-02-15
- Volume
- 88
- Issue
- 4
- Pages
- 2372-2378
- ISSN
- 0021-9606 (ISSN-L)
- 1089-7690
- OpenAlex
- W2003564103
- Cited by
- 161
- References
- 1
- FWCI
- 15.68
- Type
- journal article
- Language
- en
- Open access
- closed
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- Kahlow, M. A., Kang, T. J., & Barbara, P. F. (1988). Transient solvation of polar dye molecules in polar aprotic solvents. The Journal of Chemical Physics. https://doi.org/10.1063/1.454020
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