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The hydration of Dy3+ and Yb3+ in aqueous solution: A neutron scattering first order difference study
Open accessAbstract
The coordination of water molecules around the metal ion in acidified 1 m DyCl3, 1.0 m Dy(ClO4)3, 0.3 m Dy(ClO4)3, and 1.0 m Yb(ClO4)3 solutions in D2O have been determined by the neutron diffraction difference technique. A coordination number of eight is found for the two ions, which depends neither on the counterion, nor on the concentration. The near metal–oxygen and metal–deuterium distances are, respectively, 2.39±0.02 and 3.03±0.02 Å for dysprosium and 2.33±0.02 and 2.98±0.02 Å for ytterbium. A general discussion concerning the hydration of the lanthanide ions is given.
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Cited by
Water exchange on metal ions: experiments and simulations
Helm, L., & Merbach, A. E. (1999) · Coordination Chemistry Reviews · doi:10.1016/s0010-8545(99)90232-1 · Cited by 531
Self-citationLanthanide induced shifts and relaxation rate enhancements
Peters, J. A., Huskens, J., & Raber, D. J. (1996) · Progress in Nuclear Magnetic Resonance Spectroscopy · doi:10.1016/0079-6565(95)01026-2 · Cited by 508
Aime, S., Botta, M., Fasano, M., Marques, M. P. M., Geraldes, C. F. G. C., Pubanz, D., & Merbach, A. E. (1997) · Inorganic Chemistry · doi:10.1021/ic961364o · Cited by 368
Self-citationMechanistic Studies of Metal Aqua Ions: A Semi‐Historical Perspective
Lincoln, S. F. (2005) · Helvetica Chimica Acta · doi:10.1002/hlca.200590036 · Cited by 110
Leonarski, F., D'Ascenzo, L., & Auffinger, P. (2019) · RNA · doi:10.1261/rna.068437.118 · Cited by 39
Metadata
- Authors
- Cossy, C., Barnes, A. C., Enderby, J. E., & Merbach, A. E.
- Venue
- The Journal of Chemical Physics
- Publisher
- AIP Publishing
- Published
- 1989-03-15
- Volume
- 90
- Issue
- 6
- Pages
- 3254-3260
- ISSN
- 0021-9606 (ISSN-L)
- 1089-7690
- OpenAlex
- W56537784
- Cited by
- 168
- References
- 0
- FWCI
- 9.23
- Type
- journal article
- Language
- en
- Open access
- green
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- CoChat. (2026). Citation check: The hydration of Dy3+ and Yb3+ in aqueous solution: A neutron scattering first order difference study. https://app.cochat.ai/papers/10.1063/1.455878
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- Cossy, C., Barnes, A. C., Enderby, J. E., & Merbach, A. E. (1989). The hydration of Dy3+ and Yb3+ in aqueous solution: A neutron scattering first order difference study. The Journal of Chemical Physics. https://doi.org/10.1063/1.455878
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