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An assessment of the role of dipoles on the density-of-states function of disordered molecular solids
Abstract
The effect of permanent dipoles on the density-of-states (DOS) function of an array of hopping sites is examined by summing the contributions of individual dipoles to the total potential at a given site. For relative dipolar site concentrations ≳0.1, the DOS function is of Gaussian shape. At lower concentrations, it approaches a Lorentzian. Good agreement with literature data on the dipolar contribution to the DOS function for hole transport in molecularly doped polymers and molecular glasses differing with regard to dipole moment and concentration of dipolar moieties is found.
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Cited by
Charge Transport in Organic Semiconductors
Coropceanu, V., Cornil, J., da Silva Filho, D. A., Olivier, Y., Silbey, R., & Brédas, J.-L. (2007) · Chemical Reviews · doi:10.1021/cr050140x · Cited by 4,607
Charge-Dipole Model for the Universal Field Dependence of Mobilities in Molecularly Doped Polymers
Dunlap, D. H., Parris, P. E., & Kenkre, V. M. (1996) · Physical Review Letters · doi:10.1103/physrevlett.77.542 · Cited by 458
Device physics of organic electrochemical transistors
Friedlein, J. T., McLeod, R. R., & Rivnay, J. (2018) · Organic Electronics · doi:10.1016/j.orgel.2018.09.010 · Cited by 429
Liess, A., Arjona‐Esteban, A., Kudzus, A., Albert, J., Krause, A., Lv, A., Stolte, M., Meerholz, K., & Würthner, F. (2019) · Advanced Functional Materials · doi:10.1002/adfm.201805058 · Cited by 93
Metadata
- Authors
- Dieckmann, A., Bässler, H., & Borsenberger, P. M.
- Venue
- The Journal of Chemical Physics
- Publisher
- AIP Publishing
- Published
- 1993-11-15
- Volume
- 99
- Issue
- 10
- Pages
- 8136-8141
- ISSN
- 0021-9606 (ISSN-L)
- 1089-7690
- OpenAlex
- W2078621899
- Cited by
- 245
- References
- 0
- FWCI
- 19.75
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: An assessment of the role of dipoles on the density-of-states function of disordered molecular solids. https://app.cochat.ai/papers/10.1063/1.465640
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- Dieckmann, A., Bässler, H., & Borsenberger, P. M. (1993). An assessment of the role of dipoles on the density-of-states function of disordered molecular solids. The Journal of Chemical Physics. https://doi.org/10.1063/1.465640
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
