The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Fast responses from ‘‘slowly relaxing’’ liquids: A comparative study of the femtosecond dynamics of triacetin, ethylene glycol, and water
Abstract
We have measured the ultrafast solvent relaxation of liquid ethylene glycol, triacetin, and water by means of femtosecond polarization spectroscopy, using optical-heterodyne-detected Raman-induced Kerr-effect spectroscopy. In the viscous liquids triacetin and ethylene glycol, femtosecond relaxation processes were resolved. Not surprisingly, the femtosecond nonlinear optical response of ethylene glycol is quite similar to that of water. Using the theory of Maroncelli, Kumar, and Papazyan, we transform the pure-nuclear solvent response into a dipolar-solvation correlation function for comparison with ultrafast electron-transfer reaction rates.
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Cites
Dynamics of the dissipative two-state system
Leggett, A. J., Chakravarty, S., Dorsey, A. T., Fisher, M. P. A., Garg, A., & Zwerger, W. (1987) · Reviews of Modern Physics · doi:10.1103/revmodphys.59.1 · Cited by 5,109
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Coherent Two-Dimensional Optical Spectroscopy
Cho, M. (2008) · Chemical Reviews · doi:10.1021/cr078377b · Cited by 835
Metadata
- Authors
- Chang, Y. J., & Castner, E. W.
- Venue
- The Journal of Chemical Physics
- Publisher
- AIP Publishing
- Published
- 1993-11-15
- Volume
- 99
- Issue
- 10
- Pages
- 7289-7299
- ISSN
- 0021-9606 (ISSN-L)
- 1089-7690
- OpenAlex
- W2033919681
- Cited by
- 225
- References
- 1
- FWCI
- 9.08
- Type
- journal article
- Language
- en
- Open access
- closed
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- Chang, Y. J., & Castner, E. W. (1993). Fast responses from ‘‘slowly relaxing’’ liquids: A comparative study of the femtosecond dynamics of triacetin, ethylene glycol, and water. The Journal of Chemical Physics. https://doi.org/10.1063/1.465710
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