The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Off-resonant fifth-order nonlinear response of water and CS2: Analysis based on normal modes
Abstract
Off-resonant fifth-order nonlinear response functions of liquid water and liquid CS2 are analyzed based on two normal-mode schemes, quenched and instantaneous normal modes. It was found that the fifth-order response function is very sensitive to the mode mixing in polarization, arising from the quadratic term of polarization with respect to the different modes. The echo signal is drastically reduced by this off-diagonal mode mixing in polarization even without any rapid frequency modulation mechanism. The near absence of echo signal thus obtained for liquids is consistent with the recent experimental results for liquid CS2. The present calculation yields the different fifth-order signals for different polarization geometries, as experimentally shown by Tokmakoff and Fleming [J. Chem. Phys. 106, 2569 (1997)]. The mode mixing dynamics is investigated in terms of the bispectra of total potential energy and polarizability.
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Citations
Cites
Large local energy fluctuations in water. II. Cooperative motions and fluctuations
Ohmine, I., Tanaka, H., & Wolynes, P. G. (1988) · The Journal of Chemical Physics · doi:10.1063/1.455536 · Cited by 216
Self-citation
Cited by
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Mukamel, S. (2000) · Annual Review of Physical Chemistry · doi:10.1146/annurev.physchem.51.1.691 · Cited by 894
Coherent Two-Dimensional Optical Spectroscopy
Cho, M. (2008) · Chemical Reviews · doi:10.1021/cr078377b · Cited by 835
Metadata
- Authors
- Saito, S., & Ohmine, I.
- Venue
- The Journal of Chemical Physics
- Publisher
- AIP Publishing
- Published
- 1998-01-01
- Volume
- 108
- Issue
- 1
- Pages
- 240-251
- ISSN
- 0021-9606 (ISSN-L)
- 1089-7690
- OpenAlex
- W1553285572
- Cited by
- 160
- References
- 1
- FWCI
- 16.44
- Type
- journal article
- Language
- en
- Open access
- closed
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- Saito, S., & Ohmine, I. (1998). Off-resonant fifth-order nonlinear response of water and CS2: Analysis based on normal modes. The Journal of Chemical Physics. https://doi.org/10.1063/1.475375
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