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Perfect alignment and preferential orientation of nitrogen-vacancy centers during chemical vapor deposition diamond growth on (111) surfaces
Open accessAbstract
Synthetic diamond production is a key to the development of quantum metrology and quantum information applications of diamond. The major quantum sensor and qubit candidate in diamond is the nitrogen-vacancy (NV) color center. This lattice defect comes in four different crystallographic orientations leading to an intrinsic inhomogeneity among NV centers, which is undesirable in some applications. Here, we report a microwave plasma-assisted chemical vapor deposition diamond growth technique on (111)-oriented substrates, which yields perfect alignment (94% ± 2%) of as-grown NV centers along a single crystallographic direction. In addition, clear evidence is found that the majority (74% ± 4%) of the aligned NV centers were formed by the nitrogen being first included in the (111) growth surface and then followed by the formation of a neighboring vacancy on top. The achieved homogeneity of the grown NV centers will tremendously benefit quantum information and metrology applications.
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Ladd, T. D., Jelezko, F., Laflamme, R., Nakamura, Y., Monroe, C., & O’Brien, J. L. (2010) · Nature · doi:10.1038/nature08812 · Cited by 3,592
Quantum register based on individual electronic and nuclear spin qubits in diamond
Dutt, M. V. G., Childress, L., Jiang, L., Togan, E., Maze, J., Jelezko, F., Zibrov, A. S., Hemmer, P. R., & Lukin, M. D. (2007) · Science · doi:10.1126/science.1139831 · Cited by 1,287
Cited by
Aharonovich, I., & Neu, E. (2014) · Advanced Optical Materials · doi:10.1002/adom.201400189 · Cited by 359
Bassett, L. C., Alkauskas, A., Exarhos, A. L., & Fu, K. C. (2018) · Nanophotonics · doi:10.1515/nanoph-2019-0211 · Cited by 112
Metadata
- Authors
- Michl, J., Teraji, T., Zaiser, S., Jakobi, I., Waldherr, G., Dolde, F., Neumann, P., Doherty, M. W., Manson, N. B., Isoya, J., & Wrachtrup, J.
- Venue
- Applied Physics Letters
- Publisher
- AIP Publishing
- Published
- 2014-03-10
- Volume
- 104
- Issue
- 10
- ISSN
- 0003-6951 (ISSN-L)
- 1077-3118
- OpenAlex
- W1581200652
- Cited by
- 200
- References
- 2
- FWCI
- 8.79
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Michl, J., Teraji, T., Zaiser, S., Jakobi, I., Waldherr, G., Dolde, F., Neumann, P., Doherty, M. W., Manson, N. B., Isoya, J., & Wrachtrup, J. (2014). Perfect alignment and preferential orientation of nitrogen-vacancy centers during chemical vapor deposition diamond growth on (111) surfaces. Applied Physics Letters. https://doi.org/10.1063/1.4868128
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