Purcell enhancement of the parametric down-conversion in two-dimensional nonlinear materials
Open accessAbstract
Ultracompact nonlinear optical devices utilizing two-dimensional (2D) materials and nanostructures are emerging as important elements of photonic circuits. Integration of the nonlinear material into a subwavelength cavity or waveguide leads to a strong Purcell enhancement of the nonlinear processes and compensates for a small interaction volume. The generic feature of such devices which makes them especially challenging for analysis is strong dissipation of both the nonlinear polarization and highly confined modes of a subwavelength cavity. Here we solve a quantum-electrodynamic problem of the spontaneous and stimulated parametric down-conversion in a nonlinear quasi-2D waveguide or cavity. We develop a rigorous Heisenberg-Langevin approach which includes dissipation and fluctuations in the electron ensemble and in the electromagnetic field of a cavity on equal footing. Within a relatively simple model, we take into account the nonlinear coupling of the quantized cavity modes, their interaction with a dissipative reservoir and the outside world, amplification of thermal noise and zero-point fluctuations of the electromagnetic field, and other relevant effects. We derive closed-form analytic results for relevant quantities such as the spontaneous parametric signal power and the threshold for parametric instability. We find a strong reduction in the parametric instability threshold for 2D nonlinear materials in a subwavelength cavity and provide a comparison with conventional nonlinear photonic devices.
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All-dielectric metasurfaces exhibit much lower loss and higher damage thresholds compared to plasmonic counterparts.
“all-dielectric metasurfaces exhibit much lower loss and higher damage thresholds”
From Inverse Design of an All-Dielectric Nonlinear Polaritonic Metasurface. (2025) · cites this paper as [9]
Section IV describes a plasmonic nanocavity as having high radiative and absorption losses and says bulk transparent nonlinear devices have lower dissipation than ultracompact structures. This lends support to the loss comparison, but it does not establish that all-dielectric metasurfaces specifically have much lower loss than plasmonic metasurfaces. The paper does not compare their damage thresholds. (LLM, conf=0.78)
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Research works printed but not linked: 39
- E. M. Purcell, H. C. Torrey, and R. V. Pound, Phys. Rev. 69, 37 (1946). · DOI
- H.-B. Lin and A. J. Campillo, Phys. Rev. Lett. 73, 2440 (1994). · DOI
- P. Bermel, A. Rodriguez, J. D. Joannopoulos, and M. Soljacic, Phys. Rev. Lett. 99, 053601 (2007). · DOI
- P. Genevet, J.-P. Tetienne, E. Gatzogiannis, R. Blanchard, M. A. Kats, M. O. Scully, and F. Capasso, Nano Lett. 10, 4880 (2010). · DOI
- M. Kauranen and A. V. Zayats, Nat. Photonics 6, 737 (2012). · DOI
- M. Lapine, I. V. Shadrivov, and Y. S. Kivshar, Rev. Mod. Phys. 86, 1093 (2014). · DOI
- J. Lee et al., Nature 511, 65 (2014). · DOI
- J. Lee et al., Adv. Opt. Mater. 4, 664 (2016). · DOI
- D. Smirnova and Y. S. Kivshar, Optica 3, 1241 (2016). · DOI
- A. R. Davoyan and H. A. Atwater, Optica 5, 608 (2018). · DOI
- E. Hendry, P. J. Hale, J. Moger, A. K. Savchenko, and S. A. Mikhailov, Phys. Rev. Lett. 105, 097401 (2010). · DOI
- X. Yao and A. Belyanin, Phys. Rev. Lett. 108, 255503 (2012). · DOI
- X. Yao, M. D. Tokman, and A. Belyanin, Phys. Rev. Lett. 112, 055501 (2014). · DOI
- Y. Wang, M. Tokman, and A. Belyanin, Phys. Rev. B 94, 195442 (2016). · DOI
- L. M. Malard, T. V. Alencar, A. P. M. Barboza, K. F. Mak, and A. M. de Paula, Phys. Rev. B 87, 201401 (2013). · DOI
- H. Liu, Y. Li, Y. S. You, S. Ghimire, T. F. Heinz, and D. A. Reis, Nat. Phys. 13, 262 (2016). · DOI
- P. Alonso-Gonzlez et al., Nat. Nanotechnol. 12, 31 (2016). · DOI
- Y. Ye, Z. Wong, X. Lu, X. Ni, H. Zhu, X. Chen, Y. Wang, and X. Zhang, Nat. Photonics 9, 733 (2015). · DOI
- M. O. Scully and M. S. Zubairy, Quantum Optics (Cambridge University Press, Cambridge, 1997).
- C. Gardiner and P. Zoller, Quantum Noise (Springer-Verlag, Berlin, Heidelberg, 2004).
- M. Erukhimova and M. Tokman, Phys. Rev. A 95, 013807 (2017). · DOI
- L. Davidovich, Rev. Mod. Phys. 68, 127 (1996). · DOI
- M. Tokman, X. Yao, and A. Belyanin, Phys. Rev. Lett. 110, 077404 (2013). · DOI
- M. Erukhimova and M. Tokman, Opt. Lett. 40, 2739 (2015). · DOI
- M. Tokman and M. Erukhimova, J. Lumin. 137, 148 (2013). · DOI
- M. Tokman, Z. Long, S. AlMutairi, Y. Wang, M. Belkin, and A. Belyanin, Phys. Rev. A 97, 043801 (2018). · DOI
- V. M. Fain and Ya. I. Khanin, Quantum Electronics (The MIT Press, Cambridge, MA, 1969), Vol. 1.
- M. D. Tokman, M. A. Erukhimova, and V. V. Vdovin, Ann. Phys. 360, 571 (2015). · DOI
- M. Tokman, Y. Wang, I. Oladyshkin, A. R. Kutayiah, and A. Belyanin, Phys. Rev. B 93, 235422 (2016). · DOI
- Yu. A. Illinskii and L. V. Keldysh, Electromagnetic Response of Material Media (Springer, New York, 1994).
- M. D. Tokman and M. A. Erukhimova, Phys. Rev. E 84, 056610 (2011). · DOI
- Y. R. Shen, The Principles of Nonlinear Optics (Wiley, Hoboken, NJ, 2003).
- L. D. Landau and E. M. Lifshitz, Electrodynamics of Continuous Media (Pergamon Oxford, 1984).
- T. Low, A. Chaves, J. D. Caldwell, A. Kumar1, N. X. Fang, P. Avouris, T. F. Heinz, F. Guinea, L. Martin-Moreno, and F. Koppens, Nat. Mater. 16, 182 (2016). · DOI
- G. M. Akselrod, T. Ming, C. Argypoulos, T. B. Hoang, Y. Lin, X. Ling, D. R. Smith, J. Kong, and M. H. Mikkelsen, Nano Lett. 15, 3578 (2015). · DOI
- Y. Li, Y. Rao, K. F. Mak, Y. You, S. Wang, C. R. Dean, and T. F. Heinz, Nano Lett. 13, 3329 (2013). · DOI
- M. L. Trolle, Y.-C. Tsao, K. Pedersen, and T. G. Pedersen, Phys. Rev. B 92, 161409(R) (2015). · DOI
- J. U. Furst, D. V. Strekalov, D. Elser, A. Aiello, U. L. Andersen, Ch. Marquardt, and G. Leuchs, Phys. Rev. Lett. 105, 263904 (2010). · DOI
- V. O. Martynov, V. A. Mironov, and L. A. Smirnov, J. Phys. B: At., Mol. Opt. · DOI
Cited by
Sorted by citations
Inverse Design of an All-Dielectric Nonlinear Polaritonic Metasurface.
Stich, S., Mohajan, J., de Ceglia, D., Carletti, L., Jung, H., Karl, N., Brener, I., Rodriguez, A. W., Belkin, M. A., & Sarma, R. (2025) · ACS Nano · doi:10.1021/acsnano.4c16934 · Cited by 13 · see citing works
Self-citation
- Authors
- Tokman, M., Long, Z., AlMutairi, S., Wang, Y., Vdovin, V., Belkin, M., & Belyanin, A.
- Affiliations
- Institute of Applied Physics (RU)
- Texas A&M University (US)
- The University of Texas at Austin (US)
- Venue
- APL Photonics
- Publisher
- AIP Publishing
- Published
- 2018-12-11
- Volume
- 4
- Issue
- 3
- ISSN
- 2378-0967 (ISSN-L)
- OpenAlex
- W2900645057
- Cited by
- 16
- References
- 0
- Citations by year
- 2025: 1 · 2024: 1 · 2023: 2 · 2022: 4 · 2021: 1 · 2020: 3 · 2019: 4
- FWCI
- 0.92
- Type
- journal article
- Language
- en
- Open access
- gold
- doi.org
- Locations
- APL Photonics (publishedVersion, cc-by)
- arXiv (Cornell University) (submittedVersion)
- DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion, cc-by-sa)
- Figshare (submittedVersion, cc-by)
- arXiv (Cornell University)
- Funders
- Russian Foundation for Basic Research (17-02-00387)
- Air Force Office of Scientific Research (FA9550-15-1-0153, FA9550-17-1-0341)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Photorefractive and Nonlinear Optics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Strong Light-Matter Interactions
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Quantum optics and atomic interactions
- Keywords
- Purcell effect, parametric down-conversion, subwavelength cavities, nonlinear waveguides, energy dissipation, thermal noise, vacuum fluctuations, spontaneous parametric down-conversion, quantum electrodynamics, nonlinear optical devices
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