Cited by 2,123Free Radicals and AntioxidantsAdvanced oxidation water treatmentPhotochemistry and Electron Transfer Studies

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Reduction Potentials of One-Electron Couples Involving Free Radicals in Aqueous Solution

Wardman, Peter·1989·Journal of Physical and Chemical Reference Data

DOI 10.1063/1.555843

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Abstract

Reduction of an electron acceptor (oxidant), A, or oxidation of an electron donor (reductant), A2−, is often achieved stepwise via one-electron processes involving the couples A/A⋅− or A⋅−/A2− (or corresponding prototropic conjugates such as A/AH⋅ or AH⋅/AH2). The intermediate A⋅−(AH⋅) is a free radical. The reduction potentials of such one-electron couples are of value in predicting the direction or feasibility, and in some instances the rate constants, of many free-radical reactions. Electrochemical methods have limited applicability in measuring these properties of frequently unstable species, but fast, kinetic spectrophotometry (especially pulse radiolysis) has widespread application in this area. Tables of ca. 1200 values of reduction potentials of ca. 700 one-electron couples in aqueous solution are presented. The majority of organic oxidants listed are quinones, nitroaryl and bipyridinium compounds. Reductants include phenols, aromatic amines, indoles and pyrimidines, thiols and phenothiazines. Inorganic couples largely involve compounds of oxygen, sulfur, nitrogen and the halogens. Proteins, enzymes and metals and their complexes are excluded.

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Authors: Wardman, P.
Affiliations: Mount Vernon Hospital (GB)
Corresponding author: Wardman, Peter
ORCID: Wardman, Peter
Venue: Journal of Physical and Chemical Reference Data
Publisher: AIP Publishing
Published: 1989-10-01
Volume: 18
Issue: 4
Pages: 1637-1755
ISSN: 0047-2689 (ISSN-L)
1529-7845
DOI: 10.1063/1.555843
OpenAlex: W1979424160
Cited by: 2,123
References: 3
Citations by year: 2026: 66 · 2025: 63 · 2024: 99 · 2023: 76 · 2022: 96 · 2021: 114 · 2020: 77 · 2019: 88 · 2018: 81 · 2017: 96 · 2016: 80 · 2015: 80 · 2014: 77 · 2013: 71 · 2012: 61
FWCI: 19.63
Type: journal article
Language: en
Open access: closed
Locations: Journal of Physical and Chemical Reference Data (publishedVersion)
Topics: Physical Sciences › Chemistry › Organic Chemistry › Free Radicals and Antioxidants
Physical Sciences › Environmental Science › Water Science and Technology › Advanced oxidation water treatment
Physical Sciences › Chemistry › Physical and Theoretical Chemistry › Photochemistry and Electron Transfer Studies
Keywords: redox potential, free radicals, aqueous solutions, electron transfer, quinones, nitroaromatic compounds, phenols, aromatic amines, indole, pyrimidines, thiols, phenothiazines, inorganic oxidants, redox couples

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Reduction Potentials of One-Electron Couples Involving Free Radicals in Aqueous Solution

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