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Inhomogeneous dynamics in confined water nanodroplets
Abstract
The effect of confinement on the dynamical properties of liquid water was studied by mid-infrared ultrafast pump–probe spectroscopy on HDO:D 2 O in reverse micelles. By preparing water-containing reverse micelles of different well defined sizes, we varied the degree of geometric confinement in water nanodroplets with radii ranging from 0.2 to 4.5 nm. We find that water molecules located near the interface confining the droplet exhibit slower vibrational energy relaxation and have a different spectral absorption than those located in the droplet core. As a result, we can measure the orientational dynamics of these different types of water with high selectivity. We observe that the water molecules in the core show similar orientational dynamics as bulk water and that the water layer solvating the interface is highly immobile.
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Citations
Cites
Fluidity of water confined to subnanometre films
Raviv, U., Laurat, P., & Klein, J. (2001) · Nature · doi:10.1038/35092523 · Cited by 660
Cited by
Water as an active constituent in cell biology
Ball, P. (2008) · Chemical Reviews · doi:10.1021/cr068037a · Cited by 2,177
Analysis of Water in Confined Geometries and at Interfaces
Fayer, M. D., & Levinger, N. E. (2010) · Annual Review of Analytical Chemistry · doi:10.1146/annurev-anchem-070109-103410 · Cited by 284
Youssef, M., Pellenq, R. J.-M., & Yildiz, B. (2011) · Journal of the American Chemical Society · doi:10.1021/ja107003a · Cited by 284
Confinement or the Nature of the Interface? Dynamics of Nanoscopic Water
Moilanen, D. E., Levinger, N. E., Spry, D. B., & Fayer, M. D. (2007) · Journal of the American Chemical Society · doi:10.1021/ja073977d · Cited by 259
Finite Size Effects on Hydrogen Bonds in Confined Water
Musat, R., Renault, J. P., Candelaresi, M., Palmer, D. J., Le Caër, S., Righini, R., & Pommeret, S. (2008) · Angewandte Chemie International Edition · doi:10.1002/anie.200802630 · Cited by 54
Metadata
- Authors
- Dokter, A. M., Woutersen, S., & Bakker, H. J.
- Venue
- Proceedings of the National Academy of Sciences
- Published
- 2006-10-17
- Volume
- 103
- Issue
- 42
- Pages
- 15355-15358
- ISSN
- 0027-8424 (ISSN-L)
- 1091-6490
- OpenAlex
- W2010260586
- Cited by
- 173
- References
- 1
- FWCI
- 9.88
- Type
- journal article
- Language
- en
- Open access
- closed
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- Dokter, A. M., Woutersen, S., & Bakker, H. J. (2006). Inhomogeneous dynamics in confined water nanodroplets. Proceedings of the National Academy of Sciences. https://doi.org/10.1073/pnas.0603239103
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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