The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Regulating kinetics and thermodynamics of electrochemical nitrogen reduction with metal single-atom catalysts in a pressurized electrolyser
Open accessAbstract
Significance: The present-day industrial ammonia synthesis is overreliance on the Haber–Bosch process, yet consumes more than 1% of the global energy supply along with gigatonne greenhouse-gas emission per year. Electrochemical nitrogen reduction reaction (ENRR) offers a sustainable path to produce ammonia under mild conditions, while its efficiency achieved by far is fairly low, which requires the development of both catalysts and electrolyzers. Here, by the cooperation of densely populated metal single atoms on graphdiyne substrate with the pressurized electrocatalytic system, the kinetics and the thermodynamic driving force of ENRR are effectively regulated, leading to a record-high ammonia yield rate. This work motivates the technological and material coevolution for the ENRR toward its envisioned application.
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Cites
Anchoring zero valence single atoms of nickel and iron on graphdiyne for hydrogen evolution
Xue, Y., Huang, B., Yi, Y., Guo, Y., Zuo, Z., Li, Y., Jia, Z., Liu, H., & Li, Y. (2018) · Nature Communications · doi:10.1038/s41467-018-03896-4 · Cited by 1,011
Greatly Improving Electrochemical N 2 Reduction over TiO 2 Nanoparticles by Iron Doping
Wu, T., Zhu, X., Xing, Z., Mou, S., Li, C., Qiao, Y., Liu, Q., Luo, Y., Shi, X., Zhang, Y., et al. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201911153 · Cited by 499
Cited by
2D graphdiyne: An emerging carbon material
Fang, Y., Liu, Y., Qi, L., Xue, Y., & Li, Y. (2022) · Chemical Society Reviews · doi:10.1039/d1cs00592h · Cited by 520
Rong, C., Dastafkan, K., Wang, Y., & Zhao, C. (2023) · Advanced Materials · doi:10.1002/adma.202211884 · Cited by 361
Two-Dimensional Carbon Graphdiyne: Advances in Fundamental and Application Research
Zheng, X., Chen, S., Li, J., Wu, H., Zhang, C., Zhang, D., Chen, X., Gao, Y., He, F., Hui, L., et al. (2023) · ACS Nano · doi:10.1021/acsnano.3c03849 · Cited by 283
Metadata
- Authors
- Zou, H., Rong, W., Wei, S., Ji, Y., & Duan, L.
- Venue
- Proceedings of the National Academy of Sciences
- Published
- 2020-11-10
- Volume
- 117
- Issue
- 47
- Pages
- 29462-29468
- ISSN
- 0027-8424 (ISSN-L)
- 1091-6490
- OpenAlex
- W3103013862
- Cited by
- 174
- References
- 2
- FWCI
- 4.97
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Zou, H., Rong, W., Wei, S., Ji, Y., & Duan, L. (2020). Regulating kinetics and thermodynamics of electrochemical nitrogen reduction with metal single-atom catalysts in a pressurized electrolyser. Proceedings of the National Academy of Sciences. https://doi.org/10.1073/pnas.2015108117
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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