The DOI matches its Crossref record; 8 of the 8 references it cites were found in a registry or an index.
Controlled growth of a high selectivity interface for seawater electrolysis
Open accessAbstract
Overall seawater electrolysis is an important direction for the development of hydrogen energy conversion. The key issues include how to achieve high selectivity, activity, and stability in seawater electrolysis reactions. In this report, the heterostructures of graphdiyne-RhO x-graphdiyne (GDY/RhO x/GDY) were constructed by in situ-controlled growth of GDY on RhO x nanocrystals. A double layer interface of sp-hybridized carbon-oxide-Rhodium (sp-C∼O-Rh) was formed in this system. The microstructures at the interface are composed of active sites of sp-C∼O-Rh. The obvious electron-withdrawing surface enhances the catalytic activity with orders of magnitude, while the GDY outer of the metal oxides guarantees the stability. The electron-donating and withdrawing sp-C∼O-Rh structures enhance the catalytic activity, achieving high-performance overall seawater electrolysis with very small cell voltages of 1.42 and 1.52 V at large current densities of 10 and 500 mA cm−2 at room temperatures and ambient pressures, respectively. The compositional and structural superiority of the GDY-derived sp-C-metal-oxide active center offers great opportunities to engineer tunable redox properties and catalytic performance for seawater electrolysis and beyond. This is a typical successful example of the rational design of catalytic systems.
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Cites
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Man, I. C., Su, H., Calle‐Vallejo, F., Hansen, H. A., Martínez, J. I., Inoglu, N. G., Kitchin, J., Jaramillo, T. F., Nørskov, J. K., & Rossmeisl, J. (2011) · ChemCatChem · doi:10.1002/cctc.201000397 · Cited by 4,769
Enhancing Hydrogen Evolution Activity in Water Splitting by Tailoring Li + -Ni(OH) 2 -Pt Interfaces
Subbaraman, R., Tripkovic, D., Strmcnik, D., Chang, K.-C., Uchimura, M., Paulikas, A. P., Stamenkovic, V., & Markovic, N. M. (2011) · Science · doi:10.1126/science.1211934 · Cited by 3,135
Net-zero emissions energy systems
Davis, S. J., Lewis, N. S., Shaner, M., Aggarwal, S., Arent, D., Azevedo, I. L., Benson, S. M., Bradley, T., Brouwer, J., Chiang, Y.-M., et al. (2018) · Science · doi:10.1126/science.aas9793 · Cited by 2,391
Anchoring zero valence single atoms of nickel and iron on graphdiyne for hydrogen evolution
Xue, Y., Huang, B., Yi, Y., Guo, Y., Zuo, Z., Li, Y., Jia, Z., Liu, H., & Li, Y. (2018) · Nature Communications · doi:10.1038/s41467-018-03896-4 · Cited by 1,011
Self-citationLi, W., Liu, Y., Wu, M., Feng, X., Redfern, S. A. T., Shang, Y., Yong, X., Feng, T., Wu, K., Liu, Z., et al. (2018) · Advanced Materials · doi:10.1002/adma.201800676 · Cited by 642
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2D graphdiyne: An emerging carbon material
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Self-citationHydrogen Stabilized RhPdH 2D Bimetallene Nanosheets for Efficient Alkaline Hydrogen Evolution
Fan, J., Wu, J., Cui, X., Gu, L., Zhang, Q., Meng, F., Lei, B.-H., Singh, D. J., & Zheng, W. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.0c00218 · Cited by 225
Cited by
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Self-citationLiu, D., Wei, X., Lu, J., Wang, X., Liu, K., Cai, Y., Qi, Y., Wang, L., Ai, H., & Wang, Z. (2024) · Advanced Materials · doi:10.1002/adma.202408982 · Cited by 108
Yu, J., Li, Z., Liu, T., Zhao, S., Guan, D., Chen, D., Shao, Z., & Ni, M. (2023) · Chemical Engineering Journal · doi:10.1016/j.cej.2023.141674 · Cited by 99
Metadata
- Authors
- Gao, Y., Xue, Y., He, F., & Li, Y.
- Venue
- Proceedings of the National Academy of Sciences
- Published
- 2022-08-29
- Volume
- 119
- Issue
- 36
- Pages
- e2206946119-e2206946119
- ISSN
- 0027-8424 (ISSN-L)
- 1091-6490
- OpenAlex
- W4293485572
- Cited by
- 184
- References
- 8
- FWCI
- 7.27
- Type
- journal article
- Language
- en
- Open access
- hybrid
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