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A Generalized Biomass Pyrolysis Model Based on Superimposed Cellulose, Hemicelluloseand Liqnin Kinetics
Abstract
The pyrolysis of general biomass materials is modeled via a superposition of cellulose, hemi-cellulose and lignin kinetics. All three of the primary biomass components are modeled with multi-step kinetics involving both competetive primary pyrolysis and secondary tar decomposition reactions. Only “typical” (untreated) feedstocks are considered at atmospheric pyrolysis pressures. The kinetics scheme is then coupled to the porous particle model of Miller and Bellan (1996) along with appropriate properties and heats of reaction to provide a complete model for the pyrolysis of arbitrary biomass feedstocks and sample sizes. Comparisons with past isothermal and thermogravimetry experiments for a variety of biomass materials under both kinetically controlled and diffusion limited conditions show favorable agreement with the model predictions. In addition, discussions are provided which support the use of competetive char production kinetics over single and successive reaction schems which cannot currently be reconciled with observed pyrolysis behavior.
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Citations
Cites
CRC Handbook of Chemistry and Physics
(2014) · doi:10.1201/b17118 · Cited by 57,706
Cited by
Modeling chemical and physical processes of wood and biomass pyrolysis
DIBLASI, C. (2008) · Progress in Energy and Combustion Science · doi:10.1016/j.pecs.2006.12.001 · Cited by 1,752
Biomass pyrolysis-a review of modelling, process parameters and catalytic studies
Sharma, A., Pareek, V., & Zhang, D. (2015) · Renewable and Sustainable Energy Reviews · doi:10.1016/j.rser.2015.04.193 · Cited by 675
Volatile production from pyrolysis of cellulose, hemicellulose and lignin
Zhao, C., Jiang, E., & Chen, A. (2017) · Journal of the Energy Institute · doi:10.1016/j.joei.2016.08.004 · Cited by 458
Leng, E., Guo, Y., Chen, J., Liu, S., E, J., & Xue, Y. (2022) · Fuel · doi:10.1016/j.fuel.2021.122102 · Cited by 286
A review of thermochemical conversion of microalgae
Marcilla, A., Catalá, L., García-Quesada, J. C., Valdés, F. J., & Hernández, M. R. (2013) · Renewable and Sustainable Energy Reviews · doi:10.1016/j.rser.2013.06.032 · Cited by 202
Metadata
- Authors
- MILLER, R. S., & BELLAN, J.
- Venue
- Combustion Science and Technology
- Publisher
- Informa UK Limited
- Published
- 1997-07
- Volume
- 126
- Issue
- 1-6
- Pages
- 97-137
- ISSN
- 0010-2202 (ISSN-L)
- 1563-521X
- OpenAlex
- W1970182524
- Cited by
- 388
- References
- 1
- FWCI
- 3.09
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: A Generalized Biomass Pyrolysis Model Based on Superimposed Cellulose, Hemicelluloseand Liqnin Kinetics. https://app.cochat.ai/papers/10.1080/00102209708935670
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- MILLER, R. S., & BELLAN, J. (1997). A Generalized Biomass Pyrolysis Model Based on Superimposed Cellulose, Hemicelluloseand Liqnin Kinetics. Combustion Science and Technology. https://doi.org/10.1080/00102209708935670
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
