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Optically-heterodyne-detected optical Kerr effect (OHD-OKE): Applications in condensed phase dynamics
Abstract
The ultrafast optically-heterodyne-detected optical Kerr effect (OHD-OKE) is established as a relatively simple tool for recording the ultrafast dynamics of liquids with high temporal resolution and excellent signal-to-noise ratios. The principles and practice of the OHD-OKE method are outlined. Its application in recording the dynamics of several molecular liquids is described. The data are discussed in terms of the underlying microscopic molecular motions. Orientational motion--both librational and diffusive--is responsible for a significant fraction of the dynamics. Other potential contributions are discussed, but these are less readily assigned. The application of OHD-OKE measurements in interpreting ultrafast studies of the optical dynamics of solutions is discussed. Finally the extension of OHD-OKE methods to record the dynamics of more complex, heterogeneous, media is described.
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Dynamics of the dissipative two-state system
Leggett, A. J., Chakravarty, S., Dorsey, A. T., Fisher, M. P. A., Garg, A., & Zwerger, W. (1987) · Reviews of Modern Physics · doi:10.1103/revmodphys.59.1 · Cited by 5,109
Cited by
Turton, D. A., Hunger, J., Stoppa, A., Hefter, G., Thoman, A., Walther, M., Buchner, R., & Wynne, K. (2009) · Journal of the American Chemical Society · doi:10.1021/ja903315v · Cited by 261
Metadata
- Authors
- Smith, N. A., & Meech, S. R.
- Venue
- International Reviews in Physical Chemistry
- Publisher
- Informa UK Limited
- Published
- 2002-01
- Volume
- 21
- Issue
- 1
- Pages
- 75-100
- ISSN
- 0144-235X (ISSN-L)
- 1366-591X
- OpenAlex
- W2067685498
- Cited by
- 216
- References
- 1
- FWCI
- 8.06
- Type
- journal article
- Language
- en
- Open access
- closed
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- Smith, N. A., & Meech, S. R. (2002). Optically-heterodyne-detected optical Kerr effect (OHD-OKE): Applications in condensed phase dynamics. International Reviews in Physical Chemistry. https://doi.org/10.1080/01442350110092701
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