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Selective Hydrogenation of Ethyne in Ethene‐Rich Streams on Palladium Catalysts. Part 1. Effect of Changes to the Catalyst During Reaction
Abstract
The effect of various changes to the palladium catalyst during its stabilization in the course of the selective hydrogenation of ethyne‐ethene mixtures (formation of hydride and carbide phases and of carbonaceous deposits) was reviewed. The deposits in the form of a carbonaceous overlayer on the palladium surface create sites at which selective ethyne hydrogenation to ethene can occur. The carbonaceous deposit on the support increases the selectivity to ethane formation by increasing the rate of ethene hydrogenation on support sites (spillover of hydrogen from metal to the support surface) and by decreasing the effective diffusivity of ethyne in the pores.
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Cited by
Synthesis, Structure, Properties, and Applications of Bimetallic Nanoparticles of Noble Metals
Loza, K., Heggen, M., & Epple, M. (2020) · Advanced Functional Materials · doi:10.1002/adfm.201909260 · Cited by 499
Al13Fe4 as a low-cost alternative for palladium in heterogeneous hydrogenation
Armbrüster, M., Kovnir, K., Friedrich, M., Teschner, D., Wowsnick, G., Hahne, M., Gille, P., Szentmiklósi, L., Feuerbacher, M., Heggen, M., et al. (2012) · Nature Materials · doi:10.1038/nmat3347 · Cited by 406
Semagina, N., & Kiwi‐Minsker, L. (2009) · Catalysis Reviews · doi:10.1080/01614940802480379 · Cited by 181
Metadata
- Authors
- Borodziński, A., & Bond, G. C.
- Venue
- Catalysis Reviews
- Publisher
- Informa UK Limited
- Published
- 2006-07
- Volume
- 48
- Issue
- 2
- Pages
- 91-144
- ISSN
- 0161-4940 (ISSN-L)
- 1520-5703
- OpenAlex
- W1982636142
- Cited by
- 646
- References
- 0
- FWCI
- 6.98
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Selective Hydrogenation of Ethyne in Ethene‐Rich Streams on Palladium Catalysts. Part 1. Effect of Changes to the Catalyst During Reaction. https://app.cochat.ai/papers/10.1080/01614940500364909
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- Borodziński, A., & Bond, G. C. (2006). Selective Hydrogenation of Ethyne in Ethene‐Rich Streams on Palladium Catalysts. Part 1. Effect of Changes to the Catalyst During Reaction. Catalysis Reviews. https://doi.org/10.1080/01614940500364909
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