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An In-Situ Instrument for Speciated Organic Composition of Atmospheric Aerosols:T hermal Desorption A erosol G C/MS-FID (TAG)
Open accessAbstract
We introduce a new in-situ instrument, Thermal desorption Aerosol GC/MS-FID (TAG), capable of hourly measurements of speciated organic compounds in atmospheric aerosols. Aerosol samples are collected into a thermal desorption cell by means of humidification and inertial impaction. The sample is thermally desorbed and transferred with helium carrier gas into a gas chromatography (GC) column, with subsequent detection by both quadrupole mass spectrometer (MS) and a flame ionization detector (FID). The collection and analysis steps are automated, yielding around the clock speciation. This approach builds on the extensive body of knowledge available for quantification and source apportionment of organic aerosols from past research using filter-based GC/MS analyses, but it is the first instrument to achieve in-situ time resolved measurements for an essentially unlimited number of samples, making it possible to analyze changes in organic aerosol speciation over timescales ranging from hours to seasons.
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Cites
Aerosols, Climate, and the Hydrological Cycle
Ramanathan, V., Crutzen, P. J., Kiehl, J. T., & Rosenfeld, D. (2001) · Science · doi:10.1126/science.1064034 · Cited by 3,831
Cited by
Ulbrich, I. M., Canagaratna, M. R., Zhang, Q., Worsnop, D. R., & Jimenez, J. L. (2009) · Atmospheric Chemistry and Physics · doi:10.5194/acp-9-2891-2009 · Cited by 1,534
Formation of Urban Fine Particulate Matter
Zhang, R., Wang, G., Guo, S., Zamora, M. L., Ying, Q., Lin, Y., Wang, W., Hu, M., & Wang, Y. (2015) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00067 · Cited by 1,426
Canagaratna, M. R., Jimenez, J. L., Kroll, J. H., Chen, Q., Kessler, S. H., Massoli, P., Hildebrandt Ruiz, L., Fortner, E., Williams, L. R., Wilson, K. R., et al. (2015) · Atmospheric Chemistry and Physics · doi:10.5194/acp-15-253-2015 · Cited by 1,013
The Molecular Identification of Organic Compounds in the Atmosphere: State of the Art and Challenges
Nozière, B., Kalberer, M., Claeys, M., Allan, J., D’Anna, B., Decesari, S., Finessi, E., Glasius, M., Grgić, I., Hamilton, J. F., et al. (2015) · Chemical Reviews · doi:10.1021/cr5003485 · Cited by 656
Chemically-resolved aerosol volatility measurements from two megacity field studies
Huffman, J. A., Docherty, K. S., Aiken, A. C., Cubison, M. J., Ulbrich, I. M., DeCarlo, P. F., Sueper, D., Jayne, J. T., Worsnop, D. R., Ziemann, P. J., et al. (2009) · Atmospheric Chemistry and Physics · doi:10.5194/acp-9-7161-2009 · Cited by 334
Metadata
- Authors
- Williams, B. J., Goldstein, A. H., Kreisberg, N. M., & Hering, S. V.
- Venue
- Aerosol Science and Technology
- Publisher
- Informa UK Limited
- Published
- 2006-06
- Volume
- 40
- Issue
- 8
- Pages
- 627-638
- ISSN
- 0278-6826 (ISSN-L)
- 1521-7388
- OpenAlex
- W2116015342
- Cited by
- 234
- References
- 1
- FWCI
- 6.75
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Williams, B. J., Goldstein, A. H., Kreisberg, N. M., & Hering, S. V. (2006). An In-Situ Instrument for Speciated Organic Composition of Atmospheric Aerosols:T hermal Desorption A erosol G C/MS-FID (TAG). Aerosol Science and Technology. https://doi.org/10.1080/02786820600754631
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