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Neutron scattering studies of the model glass former ortho-terphenyl
Open accessAbstract
The van der Waals liquid ortho -terphenyl has long been used as a model system in the study of the glass transition. Motivated by mode-coupling theory, extensive experiments have been undertaken to monitor the onset of structural relaxation on microscopic time- and lengthscales. Using in particular quasielastic neutron scattering, the decay of density and tagged-particle correlations has been measured as a function of temperature, pressure and wavenumber. A consistent picture is developed, in which the mode-coupling singularity appears as a change of transport mechanism in the moderately viscous liquid, at temperatures far above the conventional (caloric) glass transition.
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Citations
Cites
Dispersion and Absorption in Dielectrics I. Alternating Current Characteristics
Cole, K. S., & Cole, R. H. (1941) · The Journal of Chemical Physics · doi:10.1063/1.1750906 · Cited by 10,152
Cited by
Thermodynamical scaling of the glass transition dynamics
Casalini, R., & Roland, C. M. (2004) · Physical Review E · doi:10.1103/physreve.69.062501 · Cited by 320
Metadata
- Authors
- Tölle, A.
- Venue
- Reports on Progress in Physics
- Publisher
- IOP Publishing
- Published
- 2001-10-24
- Volume
- 64
- Issue
- 11
- Pages
- 1473-1532
- ISSN
- 0034-4885 (ISSN-L)
- 1361-6633
- OpenAlex
- W2102807769
- Cited by
- 217
- References
- 1
- FWCI
- 5.12
- Type
- journal article
- Language
- en
- Open access
- bronze
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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