Evidence of Electron-Hole Imbalance in WTe 2 from High-Resolution Angle-Resolved Photoemission Spectroscopy
Open accessAbstract
WTe 2 has attracted a great deal of attention because it exhibits extremely large and non-saturating magnetoresistance. The underlying origin of such a giant magnetoresistance is still under debate. Utilizing laser-based angle-resolved photoemission spectroscopy with high energy and momentum resolutions, we reveal the complete electronic structure of WTe 2 . This makes it possible to determine accurately the electron and hole concentrations and their temperature dependence. We find that, with increasing the temperature, the overall electron concentration increases while the total hole concentration decreases. It indicates that the electron-hole compensation, if it exists, can only occur in a narrow temperature range, and in most of the temperature range there is an electron-hole imbalance. Our results are not consistent with the perfect electron-hole compensation picture that is commonly considered to be the cause of the unusual magnetoresistance in WTe 2 . We identify a flat band near the Brillouin zone center that is close to the Fermi level and exhibits a pronounced temperature dependence. Such a flat band can play an important role in dictating the transport properties of WTe 2 . Our results provide new insight on understanding the origin of the unusual magnetoresistance in WTe 2 .
The claims and statistics of this paper haven’t been checked yet.
Run the check — free, no account needed. It reads the open-access text and checks the sources it cites.
Integrity signals
Registry
Cites
Statistics
Claims the paper makes
The claims and statistics of this paper haven’t been checked yet.
Run the check — free, no account needed. It reads the open-access text and checks the sources it cites.
Self-check
Percentages, sums and reported differences re-computed from the paper’s own numbers.
The self-check needs the paper’s full text.
Cites
Soluyanov, A. A., Gresch, D., Wang, Z., Wu, Q., Troyer, M., Dai, X., & Bernevig, B. A. (2015) · Nature · doi:10.1038/nature15768 · Cited by 2,526 · see citing works
Self-citationQuantum spin Hall effect in two-dimensional transition metal dichalcogenides
Qian, X., Liu, J., Fu, L., & Li, J. (2014) · Science · doi:10.1126/science.1256815 · Cited by 2,053 · see citing works
Self-citationLarge, non-saturating magnetoresistance in WTe2
Ali, M. N., Xiong, J., Flynn, S., Tao, J., Gibson, Q. D., Schoop, L. M., Liang, T., Haldolaarachchige, N., Hirschberger, M., Ong, N. P., et al. (2014) · Nature · doi:10.1038/nature13763 · Cited by 1,673 · see citing works
Pan, X.-C., Chen, X., Liu, H., Feng, Y., Wei, Z., Zhou, Y., Chi, Z., Pi, L., Yen, F., Song, F., et al. (2015) · Nature Communications · doi:10.1038/ncomms8805 · Cited by 409 · see citing works
Self-citationSuperconductivity emerging from a suppressed large magnetoresistant state in tungsten ditelluride
Kang, D., Zhou, Y., Yi, W., et al. (2015) · Nature Communications · doi:10.1038/ncomms8804 · Cited by 347 · see citing works
Wu, Y., Mou, D., Jo, N. H., Sun, K., Huang, L., Bud'ko, S. L., Canfield, P. C., & Kaminski, A. (2016) · Physical Review B · doi:10.1103/physrevb.94.121113 · Cited by 326 · see citing works
Electronic Structure Basis for the Extraordinary Magnetoresistance in WTe2
Pletikosić, I., Ali, M. N., Fedorov, A. V., Cava, R. J., & Valla, T. (2014) · Physical Review Letters · doi:10.1103/physrevlett.113.216601 · Cited by 287 · see citing works
Quantum Oscillations, Thermoelectric Coefficients, and the Fermi Surface of Semimetallic WTe 2
Zhu, Z., Lin, X., Liu, J., Fauqué, B., Qian, T., Yang, C., Shi, Y., & Behnia, K. (2015) · Physical Review Letters · doi:10.1103/physrevlett.114.176601 · Cited by 255 · see citing works
Self-citationSignature of Strong Spin-Orbital Coupling in the Large Nonsaturating Magnetoresistance Material WTe2
Jiang, J. M., Tang, F., Pan, X., Liu, H., Niu, X. H., Wang, Y., Xu, D. F., Yang, H. F., Xie, B. P., Song, F., et al. (2015) · Physical Review Letters · doi:10.1103/physrevlett.115.166601 · Cited by 249 · see citing works
Temperature-Induced Lifshitz Transition in WTe 2
Wu, Y., Jo, N. H., Ochi, M., Huang, L., Mou, D., Bud’ko, S. L., Canfield, P. C., Trivedi, N., Arita, R., & Kaminski, A. (2015) · Physical Review Letters · doi:10.1103/physrevlett.115.166602 · Cited by 235 · see citing works
Wang, C., Zhang, Y., Huang, J., Nie, S., Liu, G., Liang, A., Zhang, Y., Shen, B., Liu, J., Hu, C., et al. (2016) · Physical review. B./Physical review. B · doi:10.1103/physrevb.94.241119 · Cited by 224 · see citing works
Self-citationBruno, F. Y., Tamai, A., Wu, Q. S., Cucchi, I., Barreteau, C., de la Torre, A., McKeown Walker, S., Riccò, S., Wang, Z., Kim, T. K., et al. (2016) · Physical Review B · doi:10.1103/physrevb.94.121112 · Cited by 201 · see citing works
Self-citationOn the Quantum Spin Hall Gap of Monolayer 1T′‐WTe 2
Zheng, F., Cai, C.-Y., Ge, S., Zhang, X., Liu, X., Lu, H., Zhang, Y., Qiu, J., Taniguchi, T., Watanabe, K., et al. (2016) · Advanced Materials · doi:10.1002/adma.201600100 · Cited by 179 · see citing works
Self-citationDrastic Pressure Effect on the Extremely Large Magnetoresistance in WTe2 : Quantum Oscillation Study
Cai, P. L., Hu, J., He, L., Pan, J., Hong, X., Zhang, Z., Zhang, J., Wei, J., Mao, Z. Q., & Li, S. Y. (2015) · Physical Review Letters · doi:10.1103/physrevlett.115.057202 · Cited by 173 · see citing works
Self-citationDirect visualization of a two-dimensional topological insulator in the single-layer 1T′−WTe2
Jia, Z., Song, Y., Li, X.-B., Ran, K., Lu, P., Zheng, H.-J., Zhu, X., Shi, Z., Sun, J., Wen, J., et al. (2017) · Physical review. B./Physical review. B · doi:10.1103/physrevb.96.041108 · Cited by 158 · see citing works
Hall effect in the extremely large magnetoresistance semimetal WTe2
Luo, Y., Li, H., Dai, Y., et al. (2015) · Applied Physics Letters · doi:10.1063/1.4935240 · Cited by 157 · see citing works
Layer-dependent quantum cooperation of electron and hole states in the anomalous semimetal WTe2
Das, P. K., Sante, D. D., Vobornik, I., et al. (2016) · Nature Communications · doi:10.1038/ncomms10847 · Cited by 125 · see citing works
Spin texture in type-II Weyl semimetal WTe2
Feng, B., Chan, Y., Feng, Y., Liu, R.-Y., Chou, M. Y., Kuroda, K., Yaji, K., Harasawa, A., Moras, P., Barinov, A., et al. (2016) · Physical review. B./Physical review. B · doi:10.1103/physrevb.94.195134 · Cited by 117 · see citing works
Self-citationRhodes, D. A., Das, S., Zhang, Q. R., Zeng, B., Pradhan, N. R., Kikugawa, N., Manousakis, E., & Balicas, L. (2015) · Physical Review B · doi:10.1103/physrevb.92.125152 · Cited by 87 · see citing works
Optical properties of the perfectly compensated semimetal WTe 2
Homes, C. C., Ali, M. N., & Cava, R. J. (2015) · Physical Review B · doi:10.1103/physrevb.92.161109 · Cited by 87 · see citing works
Wang, Y., Wang, K., Reutt‐Robey, J., et al. (2016) · Physical review. B./Physical review. B · doi:10.1103/physrevb.93.121108 · Cited by 62 · see citing works
Surface Fermi arc connectivity in the type-II Weyl semimetal candidate WTe 2
Sánchez‐Barriga, J., Vergniory, M. G., Evtushinsky, D. V., Aguilera, I., Varykhalov, A., Blügel, S., & Rader, O. (2016) · Physical review. B./Physical review. B · doi:10.1103/physrevb.94.161401 · Cited by 51 · see citing works
Multiple Fermi pockets revealed by Shubnikov-de Haas oscillations in WTe 2
Xiang, F., Veldhorst, M., Dou, S. X., & Wang, X. L. (2015) · Europhysics Letters (EPL) · doi:10.1209/0295-5075/112/37009 · Cited by 49 · see citing works
Dramatically decreased magnetoresistance in non-stoichiometric WTe2 crystals
Lv, Y., Zhang, B., Li, X., Pang, B., Zhang, F., Lin, D., Zhou, J. F., Yao, S., Chen, Y., Zhang, S., et al. (2016) · Scientific Reports · doi:10.1038/srep26903 · Cited by 42 · see citing works
Self-citationThree-dimensionality of the bulk electronic structure in WTe2
Wu, Y., Jo, N. H., Mou, D., Huang, L., Bud’ko, S. L., Canfield, P. C., & Kaminski, A. (2017) · Physical review. B./Physical review. B · doi:10.1103/physrevb.95.195138 · Cited by 35 · see citing works
The Effect of Dopants on the Magnetoresistance of WTe2Preprint
Flynn, S., Ali, M. N., & Cava, R. J. (2015) · arXiv (Cornell University) · doi:10.48550/arxiv.1506.07069 · Cited by 6 · see citing works
Flagged first, then by citations
Cited by
Sorted by citations
Transport of Topological Semimetals
Hu, J., Xu, S.-Y., Ni, N., & Mao, Z. (2019) · Annual Review of Materials Research · doi:10.1146/annurev-matsci-070218-010023 · Cited by 265 · see citing works
Self-citation
- Authors
- Wang, C.-L., Zhang, Y., Huang, J.-W., Liu, G.-D., Liang, A.-J., Zhang, Y.-X., Shen, B., Liu, J., Hu, C., Ding, Y., Liu, D.-F., Hu, Y., He, S.-L., Zhao, L., Yu, L., Hu, J., Wei, J., Mao, Z.-Q., Shi, Y.-G., Jia, X.-W., Zhang, F.-F., Zhang, S.-J., Yang, F., Wang, Z.-M., Peng, Q.-J., Xu, Z.-Y., Chen, C.-T., & Zhou, X.-J.
- Affiliations
- Chinese Academy of Sciences (CN)
- Tulane University (US)
- Academy of Military Transportation (CN)
- ORCID
- Zhao, Lin
- Venue
- Chinese Physics Letters
- Publisher
- IOP Publishing
- Published
- 2017-08
- Volume
- 34
- Issue
- 9
- Pages
- 097305
- ISSN
- 0256-307X (ISSN-L)
- 1741-3540
- OpenAlex
- W2752205378
- Cited by
- 18
- References
- 26
- Citations by year
- 2026: 1 · 2025: 2 · 2024: 2 · 2023: 1 · 2022: 1 · 2021: 2 · 2020: 3 · 2019: 2 · 2018: 1 · 2017: 3
- FWCI
- 1.04
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Licence
- Locations
- Chinese Physics Letters (publishedVersion)
- arXiv (Cornell University) (submittedVersion)
- arXiv (Cornell University)
- Funders
- U.S. Department of Energy (DESC0014208)
- National Natural Science Foundation of China (2016YFA0300600, 11574367, 2015CB921300)
- Chinese Academy of Sciences (XDB07020300)
- National Key Research and Development Program of China (2016YFA0300600, 2015CB921300, 2013CB921904)
- Topics
- Physical Sciences › Materials Science › Materials Chemistry › 2D Materials and Applications
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Topological Materials and Phenomena
- Physical Sciences › Materials Science › Materials Chemistry › Graphene research and applications
- Keywords
- WTe2, electron-hole compensation, giant magnetoresistance, electronic structure, electron density, hole concentration, temperature dependence, flat bands, two-dimensional transition metal dichalcogenides, transport properties
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
Are you an author, or do you see a problem with this page? Request a review