Multidimensional scattering of attosecond x-ray pulses detected by photon-coincidence
Open accessAbstract
We propose a new photon-coincidence measurement based on the time- and wavevector-resolved detection of photons generated by the scattering of multiple x-ray pulses with variable delays. The technique directly measures multipoint correlation functions of the charge density through superpositions of valence excitations which are created impulsively by the scattering process.
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Diffraction can be extended to multiple dimensions by photon coincidence measurements obtained by subjecting the molecule to sequences of pulses.
“Diffraction can be extended to multiple dimensions by photon coincidence measurements obtained by subjecting the molecule to sequences of pulses [42].”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [42]
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References 37 · Cited by 10
- Authors
- Biggs, J. D., Bennett, K., Zhang, Y., & Mukamel, S.
- Affiliations
- University of California, Irvine (US)
- Venue
- Journal of Physics B: Atomic, Molecular and Optical Physics
- Publisher
- IOP Publishing
- Published
- 2014-06-10
- Volume
- 47
- Issue
- 12
- Pages
- 124037
- ISSN
- 0953-4075 (ISSN-L)
- 1361-6455
- OpenAlex
- W2133099508
- Cited by
- 10
- References
- 37
- Citations by year
- 2018: 5 · 2017: 1 · 2015: 1 · 2014: 3
- FWCI
- 0.83
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Licence
- Locations
- Journal of Physics B Atomic Molecular and Optical Physics (publishedVersion)
- eScholarship (California Digital Library) (submittedVersion)
- Funders
- National Science Foundation (1058791, 0840513)
- U.S. Department of Energy
- National Institutes of Health
- Office of Science
- Division of Chemistry (CHE-0840513, CHE-1058791)
- Basic Energy Sciences
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Physics and Astronomy › Radiation › Advanced X-ray Imaging Techniques
- Physical Sciences › Physics and Astronomy › Radiation › X-ray Spectroscopy and Fluorescence Analysis
- Keywords
- attosecond X-ray pulses, photon coincidence, multipoint correlation functions, charge density, valence excitations, X-ray scattering, ultrafast electron dynamics
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