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Many-body theory of core holes
Abstract
An electronic Hamiltonian appropriate for describing core-hole processes is derived and its properties are discussed. Based on this Hamiltonian a many-body theory is presented, and a useful linked-cluster theorem is proven. A distinction between relaxation and correlation terms can be made in each order of the perturbation expansion. Under certain well-defined conditions the core-ionization process can be visualized as a Franck-Condon transition between two multidimensional potential-energy surfaces in an abstract bosonic space. The corresponding approximation, the boson approximation, is discussed and applied to the water molecule.
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Citations
Cited by
Simulating X-ray Spectroscopies and Calculating Core-Excited States of Molecules
Norman, P., & Dreuw, A. (2018) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00156 · Cited by 312
Core Ionization Initiates Subfemtosecond Charge Migration in the Valence Shell of Molecules
Kuleff, A. I., Kryzhevoi, N. V., Pernpointner, M., & Cederbaum, L. S. (2016) · Physical Review Letters · doi:10.1103/physrevlett.117.093002 · Cited by 98
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Metadata
- Authors
- Cederbaum, L. S., Domcke, W., & Schirmer, J.
- Venue
- Physical Review A
- Publisher
- American Physical Society (APS)
- Published
- 1980-07-01
- Volume
- 22
- Issue
- 1
- Pages
- 206-222
- ISSN
- 0556-2791 (ISSN-L)
- OpenAlex
- W2037063690
- Cited by
- 324
- References
- 0
- FWCI
- 3.84
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Many-body theory of core holes. https://app.cochat.ai/papers/10.1103/physreva.22.206
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- Cederbaum, L. S., Domcke, W., & Schirmer, J. (1980). Many-body theory of core holes. Physical Review A. https://doi.org/10.1103/physreva.22.206
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
