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Blue shift of the Mie plasma frequency in Ag clusters and particles
Abstract
Photodepletion spectroscopy is used to measure the optical activity of sputtered Ag ionic clusters with up to 70 atoms. With decreasing cluster size the giant resonance caused by collective excitation of the valence electrons shifts to higher frequencies. This blue shift is qualitatively explained in terms of a reduced s-d screening interaction in the surface region of the particles.
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Citations
Cites
Beiträge zur Optik trüber Medien, speziell kolloidaler Metallösungen
Mie, G. (1908) · Annalen der Physik · doi:10.1002/andp.19083300302 · Cited by 11,537
Cited by
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Zhu, W., Esteban, R., Borisov, A. G., Baumberg, J. J., Nordlander, P., Lezec, H. J., Aizpurua, J., & Crozier, K. B. (2016) · Nature Communications · doi:10.1038/ncomms11495 · Cited by 820
Theoretical Studies of Plasmonics using Electronic Structure Methods
Morton, S. M., Silverstein, D. W., & Jensen, L. (2011) · Chemical Reviews · doi:10.1021/cr100265f · Cited by 474
Nonlocal optical response in metallic nanostructures
Raza, S., Bozhevolnyi, S. I., Wubs, M., & Asger Mortensen, N. (2015) · Journal of Physics: Condensed Matter · doi:10.1088/0953-8984/27/18/183204 · Cited by 435
Campos, A., Troc, N., Cottancin, E., Pellarin, M., Weissker, H.-C., Lermé, J., Kociak, M., & Hillenkamp, M. (2019) · Nature Physics · doi:10.1038/s41567-018-0345-z · Cited by 253
Metadata
- Authors
- Tiggesbäumker, J., Köller, L., Meiwes-Broer, K.-H., & Liebsch, A.
- Venue
- Physical Review A
- Publisher
- American Physical Society (APS)
- Published
- 1993-09-01
- Volume
- 48
- Issue
- 3
- Pages
- R1749-R1752
- ISSN
- 0556-2791 (ISSN-L)
- 1050-2947
- 1094-1622
- OpenAlex
- W1999041388
- Cited by
- 285
- References
- 1
- FWCI
- 8.50
- Type
- journal article
- Language
- en
- Open access
- closed
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- Tiggesbäumker, J., Köller, L., Meiwes-Broer, K.-H., & Liebsch, A. (1993). Blue shift of the Mie plasma frequency in Ag clusters and particles. Physical Review A. https://doi.org/10.1103/physreva.48.r1749
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.