Generation of circularly polarized high-order harmonics by two-color coplanar field mixing

Abstract

An efficient method is investigated for the generation of circularly polarized high-order harmonics by a bichromatic laser field whose two components with frequencies $\ensuremath{\omega}$ and $2\ensuremath{\omega}$ are circularly polarized in the same plane, but rotate in opposite directions. The generation of intense harmonics by such a driving-field configuration was already confirmed by a previous experiment. With the help of both a semiclassical three-step model as well as a saddle-point analysis, the mechanism of harmonic generation in this case is elucidated and the plateau structure of the harmonic response and their cutoffs are established. The sensitivity of the harmonic yield and the polarization of the harmonics to imperfect circular polarization of the driving fields are investigated. Optimization of both the cutoff frequency and the harmonic efficiency with respect to the intensity ratio of the two components of the driving field is discussed. The electron trajectories responsible for the emission of particular harmonics are identified. Unlike the case of a linearly polarized driving field, they have a nonzero start velocity. By comparison with the driving-field configuration where the two components rotate in the same direction, the mechanism of the intense harmonic emission is further clarified. Depending on the (unknown) saturation intensity for the bichromatic field with counter-rotating polarizations, this scheme might be of practical interest not only because of the circular polarization of the produced harmonics, but also because of their production efficiency.