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Collective dipole oscillations in small silver clusters embedded in rare-gas matrices
Abstract
The optical-absorption spectra of small mass-selected ${\mathrm{Ag}}_{\mathit{N}}$ clusters (N=2--21) embedded in solid argon are measured in the energy range 2.5--6.2 eV. Investigation of a continuous range of cluster sizes reveals the size development of the photoabsorption behavior. The main features of the spectra are in agreement with predictions based on the Nilsson-Clemenger shell model. The measured photoabsorption cross sections are consistent with a sum-rule calculation involving only s electrons. In addition, the medium influence on the spectra is studied by changing the matrix gas from argon to krypton and xenon for the cluster sizes N=7, 11, 15, and 21.
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Beiträge zur Optik trüber Medien, speziell kolloidaler Metallösungen
Mie, G. (1908) · Annalen der Physik · doi:10.1002/andp.19083300302 · Cited by 11,537
Cited by
Theoretical Studies of Plasmonics using Electronic Structure Methods
Morton, S. M., Silverstein, D. W., & Jensen, L. (2011) · Chemical Reviews · doi:10.1021/cr100265f · Cited by 474
Campos, A., Troc, N., Cottancin, E., Pellarin, M., Weissker, H.-C., Lermé, J., Kociak, M., & Hillenkamp, M. (2019) · Nature Physics · doi:10.1038/s41567-018-0345-z · Cited by 253
Metadata
- Authors
- Fedrigo, S., Harbich, W., & Buttet, J.
- Venue
- Physical Review B
- Publisher
- American Physical Society (APS)
- Published
- 1993-04-15
- Volume
- 47
- Issue
- 16
- Pages
- 10706-10715
- ISSN
- 0163-1829 (ISSN-L)
- 1095-3795
- OpenAlex
- W2084446387
- Cited by
- 315
- References
- 1
- FWCI
- 4.97
- Type
- journal article
- Language
- en
- Open access
- closed
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- Fedrigo, S., Harbich, W., & Buttet, J. (1993). Collective dipole oscillations in small silver clusters embedded in rare-gas matrices. Physical Review B. https://doi.org/10.1103/physrevb.47.10706
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