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Ultrafast carrier dynamics in semiconductor quantum dots
Abstract
The dynamics of band-edge photoluminescence (PL) in CdS nanocrystals (NC's) dispersed in a glass matrix are studied with the femtosecond up-conversion technique. The time-resolved PL spectra exhibit several discrete features (three of them are in the NC energy band gap) which are not pronounced in a cw PL spectrum. The initial stage of a PL decay is governed by a depopulation of the lowest extended states due to carrier trapping (localization) on the time scale of 1 ps. The low-energy bands originating from the extended-to-localized state transitions exhibit extremely fast buildup dynamics (rise time is 400--700 fs) which is explained by the preexisting occupation of the localized states. \textcopyright{} 1996 The American Physical Society.
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Citations
Cited by
Chemistry and Properties of Nanocrystals of Different Shapes
Burda, C., Chen, X., Narayanan, R., & El-Sayed, M. A. (2005) · Chemical Reviews · doi:10.1021/cr030063a · Cited by 7,230
Electron and hole relaxation pathways in semiconductor quantum dots
Klimov, V. I., McBranch, D. W., Leatherdale, C. A., & Bawendi, M. G. (1999) · Physical Review B · doi:10.1103/physrevb.60.13740 · Cited by 686
Self-citationFemtosecond1P-to-1SElectron Relaxation in Strongly Confined Semiconductor Nanocrystals
Klimov, V. I., & McBranch, D. W. (1998) · Physical Review Letters · doi:10.1103/physrevlett.80.4028 · Cited by 503
Self-citationIntraband relaxation in CdSe quantum dots
Guyot-Sionnest, P., Shim, M., Matranga, C., & Hines, M. (1999) · Physical Review B · doi:10.1103/physrevb.60.r2181 · Cited by 393
Plasmon-Induced Hot Electron Transfer from the Au Tip to CdS Rod in CdS-Au Nanoheterostructures
Wu, K., Rodríguez-Córdoba, W. E., Yang, Y., & Lian, T. (2013) · Nano Letters · doi:10.1021/nl402730m · Cited by 334
Metadata
- Authors
- Klimov, V., Bolivar, P. H., & Kurz, H.
- Venue
- Physical Review B
- Publisher
- American Physical Society (APS)
- Published
- 1996-01-15
- Volume
- 53
- Issue
- 3
- Pages
- 1463-1467
- ISSN
- 0163-1829 (ISSN-L)
- 1095-3795
- OpenAlex
- W2014970095
- Cited by
- 193
- References
- 0
- FWCI
- 10.13
- Type
- journal article
- Language
- en
- Open access
- closed
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