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Ultrafast electron dynamics at metal surfaces: Competition between electron-phonon coupling and hot-electron transport
Abstract
An experimental scheme (double pump/reflectivity probe using femtosecond laser pulses) enables the investigation of nonequilibrium electron dynamics at metal surfaces by measuring the equilibrated surface temperature. The competition between electron-phonon coupling and hot-electron transport gives rise to a reduced equilibrated temperature when the two pump pulses overlap in time, and provides a way of accurately determining the electron-phonon coupling constant. These observations have important consequences for femtosecond photochemical investigations.
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Citations
Cited by
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Self-citationPhotochemistry on Metal Nanoparticles
Watanabe, K., Menzel, D., Nilius, N., & Freund, H.-J. (2006) · Chemical Reviews · doi:10.1021/cr050167g · Cited by 486
Laser-Induced Ultrafast Demagnetization in Ferromagnetic Metals
Zhang, G. P., & Hübner, W. (2000) · Physical Review Letters · doi:10.1103/physrevlett.85.3025 · Cited by 395
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Frischkorn, C., & Wolf, M. (2006) · Chemical Reviews · doi:10.1021/cr050161r · Cited by 349
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Metadata
- Authors
- Bonn, M., Denzler, D. N., Funk, S., Wolf, M., Wellershoff, S.-S., & Hohlfeld, J.
- Venue
- Physical Review B
- Publisher
- American Physical Society (APS)
- Published
- 2000-01-01
- Volume
- 61
- Issue
- 2
- Pages
- 1101-1105
- ISSN
- 0163-1829 (ISSN-L)
- 1095-3795
- OpenAlex
- W2061876455
- Cited by
- 220
- References
- 0
- FWCI
- 5.22
- Type
- journal article
- Language
- en
- Open access
- closed
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- Bonn, M., Denzler, D. N., Funk, S., Wolf, M., Wellershoff, S.-S., & Hohlfeld, J. (2000). Ultrafast electron dynamics at metal surfaces: Competition between electron-phonon coupling and hot-electron transport. Physical Review B. https://doi.org/10.1103/physrevb.61.1101
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