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Relative contributions to the plasmon line shape of metal nanoshells
Abstract
Nanoshells are mesoscopic particles consisting of a dielectric core coated with a metal shell, in particular gold or silver, of uniform nanometer scale thickness. This topology supports plasmon excitations with frequencies that are sensitively dependent on the relative radii of the nanoparticle's core and shell. The plasmon linewidth for this geometry is typically quite broad, nominally 100 nm or more in wavelength at plasmon resonance wavelengths in the near infrared. Several distinct physical mechanisms control the plasmon lineshape: phase retardation effects, including multipolar plasmon contributions; inhomogeneous broadening due to core and shell size distributions; and electron scattering at the shell interfaces. These mechanisms are examined in terms of their relative contributions to the plasmon line shape for nanoshells fabricated with diameters of 100--250 nm.
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Cites
Optical Constants of the Noble Metals
Johnson, P. B., & Christy, R. W. (1972) · Physical Review B · doi:10.1103/physrevb.6.4370 · Cited by 20,094
Cited by
Templated Techniques for the Synthesis and Assembly of Plasmonic Nanostructures
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Small particles, big impacts: A review of the diverse applications of nanofluids
Taylor, R., Coulombe, S., Otanicar, T., Phelan, P., Gunawan, A., Lv, W., Rosengarten, G., Prasher, R., & Tyagi, H. (2013) · Journal of Applied Physics · doi:10.1063/1.4754271 · Cited by 759
Sun, Y., Wiley, B., Li, Z.-Y., & Xia, Y. (2004) · Journal of the American Chemical Society · doi:10.1021/ja048789r · Cited by 422
Optical amplification of photothermal therapy with gold nanoparticles and nanoclusters
Khlebtsov, B., Zharov, V., Melnikov, A., Tuchin, V., & Khlebtsov, N. (2006) · Nanotechnology · doi:10.1088/0957-4484/17/20/022 · Cited by 377
Gorji, T. B., & Ranjbar, A. A. (2017) · Renewable and Sustainable Energy Reviews · doi:10.1016/j.rser.2017.01.015 · Cited by 299
Metadata
- Authors
- Westcott, S. L., Jackson, J. B., Radloff, C., & Halas, N. J.
- Venue
- Physical Review B
- Publisher
- American Physical Society (APS)
- Published
- 2002-10-31
- Volume
- 66
- Issue
- 15
- ISSN
- 0163-1829 (ISSN-L)
- 1095-3795
- OpenAlex
- W2043789526
- Cited by
- 222
- References
- 1
- FWCI
- 7.76
- Type
- journal article
- Language
- en
- Open access
- closed
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- Westcott, S. L., Jackson, J. B., Radloff, C., & Halas, N. J. (2002). Relative contributions to the plasmon line shape of metal nanoshells. Physical Review B. https://doi.org/10.1103/physrevb.66.155431
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