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Strongly coupled quantum dot-metal nanoparticle systems: Exciton-induced transparency, discontinuous response, and suppression as driven quantum oscillator effects
Abstract
We probe the transition to bistability that exists in a hybrid metal nanoparticle and semiconductor quantum dot (SQD) system when they are strongly coupled. In particular, we see a discontinuous jump in the response of the system (in both the diagonal and off-diagonal density-matrix elements) and a SQD response that is highly suppressed above resonance in this transition region. This discontinuous response and suppression arise because the SQD acts as a driven (quantum) oscillator. The phase change at resonance drastically alters the hybrid response when crossing the resonance. The study of this transition region, the discontinuity, and the suppression phenomena provides different insights into understanding this system, predicts a more complicated behavior than previously thought and corrects earlier work where the transition region was absent.
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Cites
Optical Constants of the Noble Metals
Johnson, P. B., & Christy, R. W. (1972) · Physical Review B · doi:10.1103/physrevb.6.4370 · Cited by 20,094
Yariv, A., & Moos, H. W. (1968) · American Journal of Physics · doi:10.1119/1.1974453 · Cited by 209
Cited by
Plasmon-induced resonance energy transfer for solar energy conversion
Li, J., Cushing, S. K., Meng, F., Senty, T. R., Bristow, A. D., & Wu, N. (2015) · Nature Photonics · doi:10.1038/nphoton.2015.142 · Cited by 757
Li, J., Cushing, S. K., Zheng, P., Senty, T., Meng, F., Bristow, A. D., Manivannan, A., & Wu, N. (2014) · Journal of the American Chemical Society · doi:10.1021/ja503508g · Cited by 586
Quantum Plexcitonics: Strongly Interacting Plasmons and Excitons
Manjavacas, A., García de Abajo, F. J., & Nordlander, P. (2011) · Nano Letters · doi:10.1021/nl200579f · Cited by 403
Metadata
- Authors
- Artuso, R. D., & Bryant, G. W.
- Venue
- Physical Review B
- Publisher
- American Physical Society (APS)
- Published
- 2010-11-09
- Volume
- 82
- Issue
- 19
- ISSN
- 1098-0121 (ISSN-L)
- 1550-235X
- OpenAlex
- W2010226908
- Cited by
- 235
- References
- 2
- FWCI
- 7.93
- Type
- journal article
- Language
- en
- Open access
- closed
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- Artuso, R. D., & Bryant, G. W. (2010). Strongly coupled quantum dot-metal nanoparticle systems: Exciton-induced transparency, discontinuous response, and suppression as driven quantum oscillator effects. Physical Review B. https://doi.org/10.1103/physrevb.82.195419
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