The DOI matches its Crossref record; 30 of the 30 references it cites were found in a registry or an index.
Supercooled water and the kinetic glass transition
Abstract
We present a molecular-dynamics study of the self-dynamics of water molecules in deeply supercooled liquid states. We find that the decay of single-particle dynamics correlation functions is characterized by a fast initial relaxation toward a plateau and by a region of self-similar dynamics, followed at late times by a stretched exponential decay. We interpret such results in the framework of the mode-coupling theory for supercooled liquids. We relate the apparent anomalies of the transport coefficients in water on lowering the temperature to the formation of cages and to the associated slow dynamics resulting from the presence of long-lived molecular cages. The so-called critical Angell temperature in supercooled water could thus be interpreted as kinetic glass transition temperature, relaxing the need of a thermodynamic singularity for the explanation of the anomalies of liquid water.
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Cites
Molecular dynamics with coupling to an external bath
Berendsen, H. J. C., Postma, J. P. M., van Gunsteren, W. F., DiNola, A., & Haak, J. R. (1984) · The Journal of Chemical Physics · doi:10.1063/1.448118 · Cited by 30,700
The missing term in effective pair potentials
Berendsen, H. J. C., Grigera, J. R., & Straatsma, T. P. (1987) · The Journal of Physical Chemistry · doi:10.1021/j100308a038 · Cited by 13,345
Formation of Glasses from Liquids and Biopolymers
Angell, C. A. (1995) · Science · doi:10.1126/science.267.5206.1924 · Cited by 4,799
Water: A Comprehensive Treatise
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Relaxation processes in supercooled liquids
Gotze, W., & Sjogren, L. (1992) · Reports on Progress in Physics · doi:10.1088/0034-4885/55/3/001 · Cited by 2,859
Phase behaviour of metastable water
Poole, P. H., Sciortino, F., Essmann, U., & Stanley, H. E. (1992) · Nature · doi:10.1038/360324a0 · Cited by 1,870
Self-citationMolecular Dynamics Study of Liquid Water
Rahman, A., & Stillinger, F. H. (1971) · The Journal of Chemical Physics · doi:10.1063/1.1676585 · Cited by 1,393
Kob, W., & Andersen, H. C. (1995) · Physical Review E · doi:10.1103/physreve.51.4626 · Cited by 1,329
Dynamical model of the liquid-glass transition
Leutheusser, E. (1984) · Physical Review A · doi:10.1103/physreva.29.2765 · Cited by 1,009
Perspective on the glass transition
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Cited by
How Water’s Properties Are Encoded in Its Molecular Structure and Energies
Brini, E., Fennell, C. J., Fernandez-Serra, M., Hribar-Lee, B., Lukšič, M., & Dill, K. A. (2017) · Chemical Reviews · doi:10.1021/acs.chemrev.7b00259 · Cited by 518
Relaxation and jump dynamics of water at the mica interface
Malani, A., & Ayappa, K. G. (2012) · The Journal of Chemical Physics · doi:10.1063/1.4717710 · Cited by 42
Metadata
- Authors
- Sciortino, F., Gallo, P., Tartaglia, P., & Chen, S. H.
- Venue
- Physical Review E
- Publisher
- American Physical Society (APS)
- Published
- 1996-12-01
- Volume
- 54
- Issue
- 6
- Pages
- 6331-6343
- ISSN
- 1063-651X (ISSN-L)
- 1095-3787
- OpenAlex
- W2132701172
- Cited by
- 355
- References
- 30
- FWCI
- 18.58
- Type
- journal article
- Language
- en
- Open access
- closed
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- Sciortino, F., Gallo, P., Tartaglia, P., & Chen, S. H. (1996). Supercooled water and the kinetic glass transition. Physical Review E. https://doi.org/10.1103/physreve.54.6331
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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