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Coherent Exciton–Surface-Plasmon-Polariton Interaction in Hybrid Metal-Semiconductor Nanostructures
Abstract
We report measurements of a coherent coupling between surface plasmon polaritons (SPP) and quantum well excitons in a hybrid metal-semiconductor nanostructure. The hybrid structure is designed to optimize the radiative exciton-SPP interaction which is probed by low-temperature, angle-resolved, far-field reflectivity spectroscopy. As a result of the coupling, a significant shift of approximately 7 meV and an increase in broadening by approximately 4 meV of the quantum well exciton resonance are observed. The experiments are corroborated by a phenomenological coupled-oscillator model predicting coupling strengths as large as 50 meV in structures with optimized detunings between the coupled exciton and SPP resonances. Such a strong interaction can, e.g., be used to enhance the luminescence yield of semiconductor quantum structures or to amplify SPP waves.
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Cites
Enhanced Spontaneous Emission by Quantum Boxes in a Monolithic Optical Microcavity
Gérard, J., Sermage, B., Gayral, B., Legrand, B., Costard, E., & Thierry-Mieg, V. (1998) · Physical Review Letters · doi:10.1103/physrevlett.81.1110 · Cited by 1,133
Cited by
Strong coupling between surface plasmon polaritons and emitters: a review
Törmä, P., & Barnes, W. L. (2015) · Reports on Progress in Physics · doi:10.1088/0034-4885/78/1/013901 · Cited by 1,644
Near-Field Mediated Plexcitonic Coupling and Giant Rabi Splitting in Individual Metallic Dimers
Schlather, A. E., Large, N., Urban, A. S., Nordlander, P., & Halas, N. J. (2013) · Nano Letters · doi:10.1021/nl4014887 · Cited by 537
Nanointerface Chemistry: Lattice-Mismatch-Directed Synthesis and Application of Hybrid Nanocrystals
Liu, J., & Zhang, J. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00443 · Cited by 423
Surface Plasmon Mediated Strong Exciton−Photon Coupling in Semiconductor Nanocrystals
Gómez, D. E., Vernon, K. C., Mulvaney, P., & Davis, T. J. (2010) · Nano Letters · doi:10.1021/nl903455z · Cited by 314
Metadata
- Authors
- Vasa, P., Pomraenke, R., Schwieger, S., Mazur, Y. I., Kunets, V., Srinivasan, P., Johnson, E., Kihm, J. E., Kim, D. S., Runge, E., Salamo, G., & Lienau, C.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2008-09-08
- Volume
- 101
- Issue
- 11
- Pages
- 116801-116801
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2134923522
- Cited by
- 232
- References
- 1
- FWCI
- 8.95
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: Coherent Exciton–Surface-Plasmon-Polariton Interaction in Hybrid Metal-Semiconductor Nanostructures. https://app.cochat.ai/papers/10.1103/physrevlett.101.116801
- The paper
- Vasa, P., Pomraenke, R., Schwieger, S., Mazur, Y. I., Kunets, V., Srinivasan, P., Johnson, E., Kihm, J. E., Kim, D. S., Runge, E., Salamo, G., & Lienau, C. (2008). Coherent Exciton–Surface-Plasmon-Polariton Interaction in Hybrid Metal-Semiconductor Nanostructures. Physical Review Letters. https://doi.org/10.1103/physrevlett.101.116801
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