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Ultrafast Nonlinear Optical Response of a Single Gold Nanorod near Its Surface Plasmon Resonance
Abstract
The ultrafast optical nonlinearity of an optically characterized single gold nanorod is investigated around its surface plasmon resonance, by combining a far-field spatial modulation technique with a high sensitivity pump-probe setup. The spectrally and temporally dependent response is quantitatively interpreted in terms of the bulklike optical nonlinearity enhanced by the plasmonic effect. The plasmon resonance dynamics is shown to be mostly governed by nonequilibrium electron and phonon processes. Their contributions to the nonlinear optical response of a single metal nano-object are elucidated, and the latter is connected to the nonlinearities of ensembles.
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Cites
Optical Constants of the Noble Metals
Johnson, P. B., & Christy, R. W. (1972) · Physical Review B · doi:10.1103/physrevb.6.4370 · Cited by 20,094
Cited by
Kauranen, M., & Zayats, A. V. (2012) · Nature Photonics · doi:10.1038/nphoton.2012.244 · Cited by 2,530
Ultrafast Spectroscopy: State of the Art and Open Challenges
Maiuri, M., Garavelli, M., & Cerullo, G. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.9b10533 · Cited by 460
Zhou, M., Zeng, C., Chen, Y., Zhao, S., Sfeir, M. Y., Zhu, M., & Jin, R. (2016) · Nature Communications · doi:10.1038/ncomms13240 · Cited by 266
Ultrafast Thermal Analysis of Surface Functionalized Gold Nanorods in Aqueous Solution
Huang, J., Park, J., Wang, W., Murphy, C. J., & Cahill, D. G. (2013) · ACS Nano · doi:10.1021/nn304738u · Cited by 83
Heat Transport between Au Nanorods, Surrounding Liquids, and Solid Supports
Park, J., Huang, J., Wang, W., Murphy, C. J., & Cahill, D. G. (2012) · The Journal of Physical Chemistry C · doi:10.1021/jp308130d · Cited by 57
Metadata
- Authors
- Baida, H., Mongin, D., Christofilos, D., Bachelier, G., Crut, A., Maioli, P., Del Fatti, N., & Vallée, F.
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2011-07-28
- Volume
- 107
- Issue
- 5
- Pages
- 057402-057402
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2043460153
- Cited by
- 244
- References
- 1
- FWCI
- 7.66
- Type
- journal article
- Language
- en
- Open access
- closed
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- Baida, H., Mongin, D., Christofilos, D., Bachelier, G., Crut, A., Maioli, P., Del Fatti, N., & Vallée, F. (2011). Ultrafast Nonlinear Optical Response of a Single Gold Nanorod near Its Surface Plasmon Resonance. Physical Review Letters. https://doi.org/10.1103/physrevlett.107.057402
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